Finite-size effects in single chain magnets: An experimental and theoretical study

被引:120
作者
Bogani, L
Caneschi, A
Fedi, M
Gatteschi, D
Massi, M
Novak, MA
Pini, MG
Rettori, A
Sessoli, R [1 ]
Vindigni, A
机构
[1] Univ Florence, Dipartimento Chim, I-50019 Sesto Fiorentino, Italy
[2] Univ Florence, INSTM, I-50019 Sesto Fiorentino, Italy
[3] Univ Florence, Dipartimento Fis, I-50019 Sesto Fiorentino, Italy
[4] Univ Florence, Ist Nazl Fis Nucl, I-50019 Sesto Fiorentino, Italy
[5] Univ Fed Rio de Janeiro, Inst Fis, BR-21945970 Rio De Janeiro, Brazil
[6] CNR, Ist Fis Applicata Nello Carrara, I-50019 Sesto Fiorentino, Italy
关键词
D O I
10.1103/PhysRevLett.92.207204
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The problem of finite-size effects in s=1/2 Ising systems showing slow dynamics of the magnetization is investigated introducing diamagnetic impurities in a Co2+-radical chain. The static magnetic properties have been measured and analyzed considering the peculiarities induced by the ferrimagnetic character of the compound. The dynamic susceptibility shows that an Arrhenius law is observed with the same energy barrier for the pure and the doped compounds while the prefactor decreases, as theoretically predicted. Multiple spin reversal has also been investigated.
引用
收藏
页码:207204 / 1
页数:4
相关论文
共 20 条
[1]   Glauber slow dynamics of the magnetization in a molecular Ising chain [J].
Caneschi, A ;
Gatteschi, D ;
Lalioti, N ;
Sangregorio, C ;
Sessoli, R ;
Venturi, G ;
Vindigni, A ;
Rettori, A ;
Pini, MG ;
Novak, MA .
EUROPHYSICS LETTERS, 2002, 58 (05) :771-777
[2]  
Caneschi A, 2001, ANGEW CHEM INT EDIT, V40, P1760, DOI 10.1002/1521-3773(20010504)40:9<1760::AID-ANIE17600>3.0.CO
[3]  
2-U
[4]  
CANESCHI A, 2000, DALTON T, V21, P3907
[5]   Evidence for single-chain magnet behavior in a MnIII-NiII chain designed with high spin magnetic units:: A route to high temperature metastable magnets [J].
Clérac, R ;
Miyasaka, H ;
Yamashita, M ;
Coulon, C .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2002, 124 (43) :12837-12844
[6]   PHYSICS OF THE DYNAMICAL CRITICAL EXPONENT IN ONE DIMENSION [J].
CORDERY, R ;
SARKER, S ;
TOBOCHNIK, J .
PHYSICAL REVIEW B, 1981, 24 (09) :5402-5403
[7]   CRITICAL-DYNAMICS OF THE OPEN ISING CHAIN [J].
DASILVA, JKL ;
MOREIRA, AG ;
SOARES, MS ;
BARRETO, FCS .
PHYSICAL REVIEW E, 1995, 52 (04) :4527-4528
[8]   STATIC MAGNETIC-PROPERTIES OF (CH3) 4NMNXCU1-XCL3, A QUANTUM FERROMAGNETIC CHAIN WITH CLASSICAL IMPURITIES - EXPERIMENT AND THEORY [J].
DUPAS, C ;
RENARD, JP ;
SEIDEN, J ;
CHEIKHROUHOU, A .
PHYSICAL REVIEW B, 1982, 25 (05) :3261-3272
[9]   Neel order in doped quasi-one-dimensional antiferromagnets [J].
Eggert, S ;
Affleck, I ;
Horton, MDP .
PHYSICAL REVIEW LETTERS, 2002, 89 (04) :1-047202
[10]   Ferromagnetism in one-dimensional monatomic metal chains [J].
Gambardella, P ;
Dallmeyer, A ;
Maiti, K ;
Malagoli, MC ;
Eberhardt, W ;
Kern, K ;
Carbone, C .
NATURE, 2002, 416 (6878) :301-304