Identification of air pollution sources by single aerosol particle fingerprints - micro-PIXE spectra

被引:13
作者
Wang, J
Guo, P
Li, X
Zhu, J
Reinert, T
Heitmann, J
Spemann, D
Vogt, J
Flagmeyer, RH
Butz, T
机构
[1] Chinese Acad Sci, Shanghai Inst Nucl Res, Shanghai 201800, Peoples R China
[2] Univ Leipzig, Abt Nukl Festkorperphys, Fak Phys & Geowissensch, D-04103 Leipzig, Germany
基金
中国国家自然科学基金;
关键词
single aerosol particle; nuclear microprobe; PIXE; artificial neural network;
D O I
10.1016/S0168-583X(99)00979-9
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
A new method for direct assessment of air pollution is developed by using nuclear microprobe techniques to analyse single aerosol particles (SAP). Every particle is characterized by its PIXE: spectrum which call be considered to be its fingerprint. The strategy for fingerprint classification and identification is used to trace a measured aerosol particle to its original source. Most of the particles have a size of up to 3 mu m. The particles are separately attached to a clean thin foil. The Leipzig Nanoprobe, LIPSION, is used for this study. There are two steps in the new method. First. collect samples from different sources. measure them and compile their characteristic spectra into a library. Then, assess the environmental samples by comparing their spectra with those in the library. An artificial neural network (ANN) package is used for spectrum comparison. (C) 2000 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:830 / 835
页数:6
相关论文
共 20 条
[1]   APPLICATION OF NEURAL NETWORKS THEORY TO IDENTIFY 2-DIMENSIONAL FLUORESCENCE-SPECTRA [J].
ALLANIC, AL ;
JEZEQUEL, JY ;
ANDRE, JC .
ANALYTICAL CHEMISTRY, 1992, 64 (21) :2618-2622
[2]  
[Anonymous], 1986, PARALLEL DISTRIBUTED
[3]   COMPARISON OF THE TRAINING OF NEURAL NETWORKS FOR QUANTITATIVE X-RAY-FLUORESCENCE SPECTROMETRY BY A GENETIC ALGORITHM AND BACKWARD ERROR PROPAGATION [J].
BOS, M ;
WEBER, HT .
ANALYTICA CHIMICA ACTA, 1991, 247 (01) :97-105
[4]   The Leipzig high-energy ion nanoprobe:: A report on first results [J].
Butz, T ;
Flagmeyer, RH ;
Heitman, J ;
Jamieson, DN ;
Legge, GJF ;
Lehmann, D ;
Reibetanz, U ;
Reinert, T ;
Saint, A ;
Spemann, D ;
Szymanski, R ;
Tröger, W ;
Vogt, J ;
Zhu, J .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2000, 161 :323-327
[5]  
CHARLSON RJ, 1991, TELLUS A, V43, P152, DOI 10.1034/j.1600-0870.1991.00013.x
[6]  
Chen Zemin, 1996, Nuclear Techniques, V19, P449
[7]   Elemental analysis by PIXE and other IBA techniques and their application to source fingerprinting of atmospheric fine particle pollution [J].
Cohen, DD ;
Bailey, GM ;
Kondepudi, R .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1996, 109 :218-226
[8]   Scanning proton microprobe applied to analysis of individual aerosol particles from Amazon Basin [J].
Gerab, F ;
Artaxo, P ;
Swietlicki, E ;
Pallon, J .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1998, 136 :318-323
[9]  
GRIEKEN RV, 1998, P 6 INT C NUCL MICR
[10]   Environmental applications of the LANL nuclear microprobe [J].
Hickmott, DD ;
Herrin, JM ;
Abell, R ;
George, M ;
Stimac, J ;
Gauerke, ER ;
Denniston, RF .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1997, 130 (1-4) :564-570