CMAQ/CAMx annual 2002 performance evaluation over the eastern US

Operational, diagnostic, and comparative evaluations of two one-atmosphere regional models were performed for the full calendar year 2002 in support of regional haze regulatory applications in the eastern US. Using consistent emissions, meteorological and air quality data sets, the community multi-scale air quality and comprehensive air quality model with extensions models were exercised on a nested 36/12 km grid system and evaluated across a broad range of time and space scales for numerous gas-phase and fine particulate species derived from routine and research-grade ambient measurements at six monitoring networks. Performance by both models for speciated fine particulate matter (PM) across the eastern US SO42-) ranged from quite good (e.g., 4 to poor (e.g., soil). For most species, model bias was higher in the winter and lower (usually negative) in the summer suggesting potential issues related to vertical mixing (e.g., too little in winter), temporal allocation of emissions, and/or other model science processes or inputs. These results may be used to (a) guide one-atmosphere model refinements, (b) improve data input preparation procedures, (c) evaluate methods for rigorous, stressful performance testing, and (d) clarify the uncertainty in model estimates for regional haze and PM2.5 control strategy programs. (c) 2006 Elsevier Ltd. All rights reserved.