Field-driven solid-on-solid interfaces moving under a stochastic Arrhenius dynamics:: Effects of the barrier height

被引:5
作者
Buendia, G. M. [1 ]
Rikvold, P. A.
Kolesik, M.
机构
[1] Univ Simon Bolivar, Dept Phys, Caracas 1080, Venezuela
[2] Florida State Univ, Sch Computat Sci, Dept Phys, Tallahassee, FL 32306 USA
[3] Florida State Univ, Ctr Mat Res & Technol, Tallahassee, FL 32306 USA
[4] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA
[5] Slovak Acad Sci, Inst Phys, Bratislava, Slovakia
[6] Univ Arizona, Ctr Opt Sci, Tucson, AZ 85721 USA
来源
JOURNAL OF MOLECULAR STRUCTURE-THEOCHEM | 2006年 / 769卷 / 1-3期
基金
美国国家科学基金会;
关键词
interface structure; Arrhenius dynamics; Monte Carlo simulation;
D O I
10.1016/j.theochem.2006.04.031
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We present analytical results and kinetic Monte Carlo simulations for the mobility and microscopic structure of solid-on-solid (SOS) interfaces driven far from equilibrium by an external force, such as an applied field or (electro)chemical potential difference. The interfaces evolve under a specific stochastic dynamics with a local energy barrier (an Arrhenius dynamics), known as the transition dynamics approximation (TDA). We calculate the average height of steps on the interface, the average interface velocity, and the skewness of the interface as functions of the driving force and the height of the energy barrier. We find that the microscopic interface structure depends quite strongly on the barrier height. As the barrier becomes higher, the local interface width decreases and the skewness increases, suggesting increasing short-range correlations between the step heights. (c) 2006 Elsevier B.V. All rights reserved.
引用
收藏
页码:207 / 210
页数:4
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