Macroscopic size effects in second harmonic generation from Si(111) coated by thin oxide films: The role of optical casimir nonlocality

被引:16
作者
Aktsipetrov, OA [1 ]
Fedyanin, AA [1 ]
Mishina, ED [1 ]
Nikulin, AA [1 ]
Rubtsov, AN [1 ]
vanHasselt, CW [1 ]
Devillers, MAC [1 ]
Rasing, T [1 ]
机构
[1] CATHOLIC UNIV NIJMEGEN, INST MAT RES, NL-6525 ED NIJMEGEN, NETHERLANDS
关键词
D O I
10.1103/PhysRevLett.78.46
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Optical second harmonic generation from Si(111)-SiO2 interface shows a strong nonmonotonic dependence on the oxide thickness between 1 and 300 nm. The Brewster angle of incidence, pin, p-out combination of polarizations and strong, uniform suppression of this effect by near-index matching fluid exclude trivial multiple reflections and microscopic interface effects. The observation can be interpreted to originate from the optical (Casimir) nonlocality stemming from the thickness-dependent electron-electron interaction via virtual photons of the quantized electromagnetic field.
引用
收藏
页码:46 / 49
页数:4
相关论文
共 24 条
[1]  
Aktsipetrov O. A., 1984, Soviet Physics - Doklady, V29, P37
[2]  
AKTSIPETROV OA, 1986, ZH EKSP TEOR FIZ, V64, P167
[3]  
BARASH YS, 1989, DIELECTRIC FUNCTION, P389
[4]   A maritime analogy of the Casimir effect [J].
Boersma, SL .
AMERICAN JOURNAL OF PHYSICS, 1996, 64 (05) :539-541
[5]   THE INFLUENCE OF RETARDATION ON THE LONDON-VANDERWAALS FORCES [J].
CASIMIR, HBG ;
POLDER, D .
PHYSICAL REVIEW, 1948, 73 (04) :360-372
[6]   IDENTIFICATION OF STRAINED SILICON LAYERS AT SI-SIO2 INTERFACES AND CLEAN SI SURFACES BY NONLINEAR-OPTICAL SPECTROSCOPY [J].
DAUM, W ;
KRAUSE, HJ ;
REICHEL, U ;
IBACH, H .
PHYSICAL REVIEW LETTERS, 1993, 71 (08) :1234-1237
[7]   SURFACE 2ND-HARMONIC STUDIES OF SI(111)/ELECTROLYTE AND SI(111)/SIO2/ELECTROLYTE INTERFACES [J].
FISCHER, PR ;
DASCHBACH, JL ;
RICHMOND, GL .
CHEMICAL PHYSICS LETTERS, 1994, 218 (03) :200-205
[8]   LOCAL AND NONLOCAL SURFACE NONLINEARITIES FOR SURFACE OPTICAL 2ND-HARMONIC GENERATION [J].
GUYOTSIONNEST, P ;
SHEN, YR .
PHYSICAL REVIEW B, 1987, 35 (09) :4420-4426
[9]   STUDY OF SYMMETRY AND DISORDERING OF SI(111)-7X7 SURFACES BY OPTICAL 2ND HARMONIC-GENERATION [J].
HEINZ, TF ;
LOY, MMT ;
THOMPSON, WA .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 1985, 3 (05) :1467-1470
[10]  
HEINZ TF, 1991, NONLINEAR SURFACE EL, P355