Multiresponse optimization based on the desirability function for a pervaporation process for producing anhydrous ethanol

被引:8
作者
Nguyen, Hun Hieu [1 ]
Jang, Namjin [1 ]
Choi, Soo Myoung [1 ]
机构
[1] Chonbuk Natl Univ, Sch Semicond & Chem Engn, Jeonju 561756, South Korea
关键词
Multiresponse Optimization; Overall Desirability Function; Central Composite Rotatable Design; Response Surface Methodology; Pervaporation; COMPOSITE MEMBRANES; WATER MIXTURES; DEHYDRATION; ISOPROPANOL; SEPARATION; MODEL;
D O I
10.1007/s11814-009-0001-5
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A pervaporation process for producing anhydrous ethanol from industrial ethyl alcohol (95% v/v) was performed with a commercial PVA/PAN membrane. A central composite rotatable experimental design together with response surface methodology was implemented for studying and modeling the influence of operating conditions in terms of the temperature and the flow rate of the feed on the pervaporation performance, namely, the permeate flux and the separation factor. To obtain a trade-off between the permeate flux and the separation factor, a method for simultaneous optimization of multiple responses based on an overall desirability function was used. The optimization resulted in a feed temperature of 66 degrees C and a feed flow rate of 42 L/h. These operating conditions are expected to respond with a permeate flux of 0.107 kg/m(2)h and a separation factor of 40, which correspond to a satisfactory overall desirability.
引用
收藏
页码:1 / 6
页数:6
相关论文
共 19 条
[1]  
AMINABHAVI TM, 1994, J MACROMOL SCI R M C, VC34, P139
[2]  
Fuller D., 1998, DESIRABILITY FUNCTIO
[3]  
HSIUNG CS, 2001, J MEMBRANE SCI, V193, P59
[4]  
HSU CS, 2004, W J APPL POLYM SCI, V87, P2158
[5]  
Huang R.Y.M., 1991, PERVAPORATION MEMBRA, p.111
[6]   Multilayer poly(vinyl alcohol)-zeolite 4A composite membranes for ethanol dehydration by means of pervaporation [J].
Huang, Zhen ;
Shi, Yan ;
Wen, Rui ;
Guo, Yu-Hua ;
Su, Jun-Feng ;
Matsuura, T. .
SEPARATION AND PURIFICATION TECHNOLOGY, 2006, 51 (02) :126-136
[7]   Pervaporation dehydration of ethanol-water mixtures with chitosan/hydroxyethylcellulose (CS/HEC) composite membranes I. Effect of operating conditions [J].
Jiraratananon, R ;
Chanachai, A ;
Huang, RYM ;
Uttapap, D .
JOURNAL OF MEMBRANE SCIENCE, 2002, 195 (02) :143-151
[8]  
Lazic Z.R., 2004, DESIGN EXPT CHEM ENG
[9]   Pervaporation of ionically surface crosslinked chitosan composite membranes for water-alcohol mixtures [J].
Lee, YM ;
Nam, SY ;
Woo, DJ .
JOURNAL OF MEMBRANE SCIENCE, 1997, 133 (01) :103-110
[10]   Hydrophobic pervaporation for environmental applications: Process optimization and integration [J].
Lipnizki, F ;
Field, RW .
ENVIRONMENTAL PROGRESS, 2002, 21 (04) :265-272