The vibrational approach to determine molecular nonlinearities: What do we learn from the method and the data?

被引:8
作者
DelZoppo, M
Castiglioni, C
Zuliani, P
Zerbi, G
机构
关键词
infrared and Raman spectroscopy; non linear optical methods; polyacetylene and derivatives;
D O I
10.1016/S0379-6779(97)80145-2
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
It is shown that molecular non linear optical properties can be measured with the vibrational infrared and Raman spectra. Correlations between optical non linearities and structural features are discussed.
引用
收藏
页码:1043 / 1046
页数:4
相关论文
共 23 条
[1]   VERY LARGE QUADRATIC NONLINEARITIES IN SOLUTION OF 2 PUSH-PULL POLYENE SERIES - EFFECT OF THE CONJUGATION LENGTH AND OF THE END GROUPS [J].
BARZOUKAS, M ;
BLANCHARDDESCE, M ;
JOSSE, D ;
LEHN, JM ;
ZYSS, J .
CHEMICAL PHYSICS, 1989, 133 (02) :323-329
[2]   MOLECULAR VIBRATIONAL AND ROTATIONAL MOTION IN STATIC AND DYNAMIC ELECTRIC-FIELDS [J].
BISHOP, DM .
REVIEWS OF MODERN PHYSICS, 1990, 62 (02) :343-374
[3]   CHAIN-LENGTH DEPENDENCE OF THE QUADRATIC HYPERPOLARIZABILITY OF PUSH-PULL POLYENES AND CAROTENOIDS - EFFECT OF END-GROUPS AND CONJUGATION PATH [J].
BLANCHARDDESCE, M ;
LEHN, JM ;
BARZOUKAS, M ;
LEDOUX, I ;
ZYSS, J .
CHEMICAL PHYSICS, 1994, 181 (1-2) :281-289
[4]   LARGE QUADRATIC HYPERPOLARIZABILITIES WITH DONOR-ACCEPTOR POLYENES FUNCTIONALIZED WITH STRONG DONORS - COMPARISON WITH DONOR-ACCEPTOR DIPHENYLPOLYENES [J].
BLANCHARDDESCE, M ;
RUNSER, C ;
FORT, A ;
BARZOUKAS, M ;
LEHN, JM ;
BLOY, V ;
ALAIN, V .
CHEMICAL PHYSICS, 1995, 199 (2-3) :253-261
[5]   VIBRATIONAL RAMAN-SPECTROSCOPY OF POLYCONJUGATED ORGANIC OLIGOMERS AND POLYMERS [J].
CASTIGLIONI, C ;
DELZOPPO, M ;
ZERBI, G .
JOURNAL OF RAMAN SPECTROSCOPY, 1993, 24 (08) :485-494
[6]   RELAXATION CONTRIBUTION TO HYPERPOLARIZABILITY - A SEMICLASSICAL MODEL [J].
CASTIGLIONI, C ;
GUSSONI, M ;
DELZOPPO, M ;
ZERBI, G .
SOLID STATE COMMUNICATIONS, 1992, 82 (01) :13-17
[7]   Molecular first hyperpolarizability of push-pull polyenes: Relationship between electronic and vibrational contribution by a two-state model [J].
Castiglioni, C ;
DelZoppo, M ;
Zerbi, G .
PHYSICAL REVIEW B, 1996, 53 (20) :13319-13325
[8]   EXPERIMENTAL MOLECULAR HYPERPOLARIZABILITIES FROM VIBRATIONAL-SPECTRA IN SYSTEMS WITH LARGE ELECTRON-PHONON COUPLING [J].
CASTIGLIONI, C ;
DELZOPPO, M ;
ZULIANI, P ;
ZERBI, G .
SYNTHETIC METALS, 1995, 74 (02) :171-177
[9]  
Chemia D. S., 1987, Nonlinear optical properties of organic molecules and crystals
[10]  
DelZoppo M, 1996, ADV MATER, V8, P345