The ID03 surface diffraction beamline for in-situ and real-time X-ray investigations of catalytic reactions at surfaces

被引：49

作者：

Balmes, O. ^{[1
]}

van Rijn, R. ^{[1
,2
]}

Wermeille, D. ^{[1
]}

Resta, A. ^{[1
]}

Petit, L. ^{[1
]}

Isern, H. ^{[1
]}

Dufrane, T. ^{[1
]}

Felici, R. ^{[1
]}

机构：

[1] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France

[2] Leiden Univ, Kamerlingh Onnes Lab, NL-2300 RA Leiden, Netherlands

来源：

CATALYSIS TODAY | 2009年 / 145卷 / 3-4期

关键词：

Catalysis; Surface X-ray diffraction; In-situ methods; Time resolved; CO oxidation; ANOMALOUS-FINE-STRUCTURE; SCATTERING; REFLECTION; PRESSURE;

D O I：

10.1016/j.cattod.2009.02.008

中图分类号：

O69 [应用化学];

学科分类号：

081704 ;

摘要：

In this article, we present the current capabilities of the ID03 surface diffraction beamline for the characterisation of catalytic surfaces under reaction. The weak interaction of X-rays with matter makes it possible to design reactor set-ups which can sustain high temperatures and atmospheric pressures while probing the sample reactivity, structure and morphology with surface sensitive X-ray techniques. A few examples are presented as an illustration of the current capabilities. (C) 2009 Elsevier B.V. All rights reserved.

引用

页码：220 / 226

页数：7

共 26 条

[1] Hydrogenation of carbon monoxide on Ni(111) investigated with surface X-ray diffraction at atmospheric pressure [J].

Ackermann, M ;

Robach, O ;

Walker, C ;

Quiros, C ;

Isern, H ;

Ferrer, S .

SURFACE SCIENCE, 2004, 557 (1-3) :21-30

[2] Structure and reactivity of surface oxides on Pt(110) during catalytic CO oxidation [J].

Ackermann, MD ;

Pedersen, TM ;

Hendriksen, BLM ;

Robach, O ;

Bobaru, SC ;

Popa, I ;

Quiros, C ;

Kim, H ;

Hammer, B ;

Ferrer, S ;

Frenken, JWM .

PHYSICAL REVIEW LETTERS, 2005, 95 (25)

[3]

ACKERMANN MD, THESIS U LEIDEN NETH

[4] Resonant atomic scattering factor theory: A multiple scattering approach [J].

Benfatto, M ;

Felici, R .

PHYSICAL REVIEW B, 2001, 64 (11)

[5] Ultrahigh vacuum high pressure chamber for surface x-ray diffraction experiments [J].

Bernard, P ;

Peters, K ;

Alvarez, J ;

Ferrer, S .

REVIEW OF SCIENTIFIC INSTRUMENTS, 1999, 70 (02) :1478-1480

[6] MOLECULAR-BEAM INVESTIGATION OF CATALYTIC-OXIDATION OF CO ON PD (111) [J].

ENGEL, T ;

ERTL, G .

JOURNAL OF CHEMICAL PHYSICS, 1978, 69 (03) :1267-1281

[7] SURFACE-STRUCTURE DETERMINATION BY X-RAY-DIFFRACTION [J].

FEIDENHANSL, R .

SURFACE SCIENCE REPORTS, 1989, 10 (03) :105-188

[8]

Gabor D., 1999, Principles of optics

[9] Sensitivity of catalysis to surface structure: The example of CO oxidation on Rh under realistic conditions [J].

Gustafson, J. ;

Westerstroem, R. ;

Mikkelsen, A. ;

Torrelles, X. ;

Balmes, O. ;

Bovet, N. ;

Andersen, J. N. ;

Baddeley, C. J. ;

Lundgren, E. .

PHYSICAL REVIEW B, 2008, 78 (04)

[10] X-RAY INTERACTIONS - PHOTOABSORPTION, SCATTERING, TRANSMISSION, AND REFLECTION AT E=50-30,000 EV, Z=1-92 [J].

HENKE, BL ;

GULLIKSON, EM ;

DAVIS, JC .

ATOMIC DATA AND NUCLEAR DATA TABLES, 1993, 54 (02) :181-342

← 1 2 3 →