Berry-phase oscillations of the kondo effect in single-molecule magnets

被引:112
作者
Leuenberger, Michael N. [1 ]
Mucciolo, Eduardo R.
机构
[1] Univ Cent Florida, Nanosci Technol Ctr, Orlando, FL 32826 USA
[2] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.97.126601
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We show that it is possible to topologically induce or quench the Kondo resonance in the conductance of a single-molecule magnet (S > 1/2) strongly coupled to metallic leads. This can be achieved by applying a magnetic field perpendicular to the molecule easy axis and works for both full- and half-integer spin cases. The effect is caused by the Berry-phase interference between two quantum tunneling paths of the molecule's spin. We have calculated the renormalized Berry-phase oscillations of the Kondo peaks as a function of the transverse magnetic field as well as the conductance of the molecule by means of the poor man's scaling method. We propose to use a new variety of the single-molecule magnet Ni-4 for the experimental observation of this phenomenon.
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页数:4
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共 29 条
[1]   POOR MANS DERIVATION OF SCALING LAWS FOR KONDO PROBLEM [J].
ANDERSON, PW .
JOURNAL OF PHYSICS PART C SOLID STATE PHYSICS, 1970, 3 (12) :2436-&
[2]   EXCHANGE MODEL OF ZERO-BIAS TUNNELING ANOMALIES [J].
APPELBAUM, JA .
PHYSICAL REVIEW, 1967, 154 (03) :633-+
[3]   Inelastic neutron scattering study of electron reduction in Mn12 derivatives [J].
Basler, R ;
Sieber, A ;
Chaboussant, G ;
Güdel, HU ;
Chakov, NE ;
Soler, M ;
Christou, G ;
Desmedt, A ;
Lechner, R .
INORGANIC CHEMISTRY, 2005, 44 (03) :649-653
[4]   Single-molecule magnets:: Structural characterization, magnetic properties, and 19F NMR spectroscopy of a Mn12 family spanning three oxidation levels [J].
Chakov, NE ;
Soler, M ;
Wernsdorfer, W ;
Abboud, KA ;
Christou, G .
INORGANIC CHEMISTRY, 2005, 44 (15) :5304-5321
[5]   QUANTUM TUNNELING OF MAGNETIZATION IN SMALL FERROMAGNETIC PARTICLES [J].
CHUDNOVSKY, EM ;
GUNTHER, L .
PHYSICAL REVIEW LETTERS, 1988, 60 (08) :661-664
[6]   A tunable Kondo effect in quantum dots [J].
Cronenwett, SM ;
Oosterkamp, TH ;
Kouwenhoven, LP .
SCIENCE, 1998, 281 (5376) :540-544
[7]   Magnetic quantum tunneling in the single-molecule magnet Mn12-acetate [J].
del Barco, E ;
Kent, AD ;
Hill, S ;
North, JM ;
Dalal, NS ;
Rumberger, EM ;
Hendrickson, DN ;
Chakov, N ;
Christou, G .
JOURNAL OF LOW TEMPERATURE PHYSICS, 2005, 140 (1-2) :119-174
[8]   Macroscopic measurement of resonant magnetization tunneling in high-spin molecules [J].
Friedman, JR ;
Sarachik, MP ;
Tejada, J ;
Ziolo, R .
PHYSICAL REVIEW LETTERS, 1996, 76 (20) :3830-3833
[9]   TOPOLOGICALLY QUENCHED TUNNEL SPLITTING IN SPIN SYSTEMS WITHOUT KRAMERS DEGENERACY [J].
GARG, A .
EUROPHYSICS LETTERS, 1993, 22 (03) :205-210
[10]  
Glazman LI, 2005, LES HOUCH S, V81, P427