Enhancement of Pairing Interaction and Magnetic Fluctuations toward a Band Insulator in an Electron-Doped LixZrNCl Superconductor

被引:50
作者
Kasahara, Yuichi [1 ]
Kishiume, Tsukasa [1 ]
Takano, Takumi [1 ]
Kobayashi, Katsuki [1 ]
Matsuoka, Eiichi [2 ]
Onodera, Hideya [2 ]
Kuroki, Kazuhiko [3 ]
Taguchi, Yasujiro [4 ]
Iwasa, Yoshihiro [1 ,5 ]
机构
[1] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan
[2] Tohoku Univ, Dept Phys, Sendai, Miyagi 9808578, Japan
[3] Univ Electrocommun, Dept Appl Phys & Chem, Tokyo 1828585, Japan
[4] RIKEN, ASI, CMRG, Wako, Saitama 3510198, Japan
[5] Japan Sci & Technol Corp, CREST, Kawaguchi, Saitama 3320012, Japan
关键词
NITRIDE CHLORIDE; HAFNIUM NITRIDE; ZIRCONIUM; SYSTEMS; STATE; HEAT;
D O I
10.1103/PhysRevLett.103.077004
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The doping dependence of specific heat and magnetic susceptibility has been investigated for LixZrNCl superconductors derived from a band insulator. As the carrier concentration is decreased, the anisotropy of superconducting gap changes from highly anisotropic to almost isotropic. It was also found that, upon reducing carrier density, the superconducting coupling strength and the magnetic susceptibility are concomitantly enhanced in parallel with T-c, while the density of states at the Fermi level is kept almost constant. Theoretical calculations taking into account the on-site Coulomb interaction reproduced the experimental results, suggesting a possible pairing mediated by magnetic fluctuations, even in the doped band insulators.
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页数:4
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