Analysis of nonlinear optical contributions to temporally two-dimensional Raman scattering

被引：34

作者：

Steffen, T

Duppen, K

机构：

[1] Department of Chemical Physics, Materials Science Center, University of Groningen

来源：

CHEMICAL PHYSICS LETTERS | 1997年 / 273卷 / 1-2期

关键词：

D O I：

10.1016/S0009-2614(97)00583-6

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Temporally two-dimensional impulsive stimulated Raman scattering can be obscured by various artefacts such as interfering or sequential third-order processes, scattering due to hyperpolarizabilities, and higher-order Bragg diffraction. These effects can modify the observed signals, depending on the employed beam configuration. However, they cannot explain the observed discrepancies between current theories and experimental results for neat carbon disulfide. (C) 1997 Elsevier Science B.V.

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页码：47 / 54

页数：8

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