Origin of the complex dielectric relaxation spectra of molecular glass formers -: art. no. 174201

被引:17
作者
Bermejo, FJ
Howells, WS
Jiménez-Ruiz, M
González, MA
Price, DL
Saboungi, ML
Cabrillo, C
机构
[1] Univ Basque Country, Dept Elect & Elect, Bilbao 48080, Spain
[2] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England
[3] CSIC, Inst Estructura Mat, E-28006 Madrid, Spain
[4] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France
[5] CNRS, Ctr Rech Mat Haute Temp, F-45071 Orleans, France
[6] Argonne Natl Lab, Argonne, IL 60439 USA
[7] Univ Orleans, CNRS, Ctr Rech Mat Divisee, F-45071 Orleans 2, France
关键词
D O I
10.1103/PhysRevB.69.174201
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The origin of the three broad bands appearing in the dielectric spectra of molecular glass formers is tracked down to microscopic scales by means of neutron-scattering and molecular-dynamics simulations. Three distinct regimes are also seen in the neutron quasielastic spectrum and are shown to arise from well-separated time regions appearing in the single-particle dipole autocorrelation function derived from simulations.
引用
收藏
页码:174201 / 1
页数:7
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