The energetics of oxide surfaces by quantum Monte Carlo

被引:36
作者
Alfe, D.
Gillan, M. J.
机构
[1] UCL, Dept Earth Sci, London WC1E 6BT, England
[2] UCL, Dept Phys & Astron, London WC1E 6BT, England
[3] UCL, London Ctr Nanotechnol, London WC1E 6BT, England
关键词
D O I
10.1088/0953-8984/18/35/L01
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Density functional theory (DFT) is widely used in surface science, but for some properties the predictions depend strongly on the approximation used for exchange-correlation energy. We note recent suggestions that the widely used generalized gradient approximation (GGA) is inferior to the local density approximation (LDA) for the surface formation energy sigma of both transition metals and oxides. We report quantum Monte Carlo calculations of s for the MgO(001) surface which support the accuracy of LDA for this case, and indicate that GGA is too low by similar to 30%. We point out the potentially important implications of this result for nanoscience modelling.
引用
收藏
页码:L435 / L440
页数:6
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