g-C3N4-Based Photocatalysts for Hydrogen Generation

被引:1169
作者
Cao, Shaowen [1 ]
Yu, Jiaguo [1 ,2 ]
机构
[1] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China
[2] King Abdulaziz Univ, Fac Sci, Jeddah 21589, Saudi Arabia
来源
JOURNAL OF PHYSICAL CHEMISTRY LETTERS | 2014年 / 5卷 / 12期
基金
中国博士后科学基金;
关键词
GRAPHITIC CARBON NITRIDE; ARTIFICIAL PHOTOSYNTHESIS; EVOLUTION; SEMICONDUCTORS; WATER; NANOSHEETS; HETEROSTRUCTURES; PHOTOREACTIVITY; CATALYSTS; GROWTH;
D O I
10.1021/jz500546b
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Graphitic carbon nitride (g-C3N4)-based photocatalysts have attracted dramatically increasing interest in the area of visible-light-induced photocatalytic hydrogen generation due to the unique electronic band structure and high thermal and chemical stability of g-C3N4. This Perspective summarizes the recent significant advances on designing high-performance g-C3N4-based photocatalysts for hydrogen generation under visible-light irradiation. The rational strategies such as nanostructure design, band gap engineering, dye sensitization, and heterojunction construction are described. Finally, this Perspective highlights the ongoing challenges and opportunities for the future development of g-C3N4-based photocatalysts in the exciting research area.
引用
收藏
页码:2101 / 2107
页数:7
相关论文
共 51 条
[31]   Polymeric Graphitic Carbon Nitride for Heterogeneous Photocatalysis [J].
Wang, Xinchen ;
Blechert, Siegfried ;
Antonietti, Markus .
ACS CATALYSIS, 2012, 2 (08) :1596-1606
[32]   Polymer Semiconductors for Artificial Photosynthesis: Hydrogen Evolution by Mesoporous Graphitic Carbon Nitride with Visible Light [J].
Wang, Xinchen ;
Maeda, Kazuhiko ;
Chen, Xiufang ;
Takanabe, Kazuhiro ;
Domen, Kazunari ;
Hou, Yidong ;
Fu, Xianzhi ;
Antonietti, Markus .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (05) :1680-+
[33]  
Wang XC, 2009, NAT MATER, V8, P76, DOI [10.1038/nmat2317, 10.1038/NMAT2317]
[34]   Carbon nitride nanosheets for photocatalytic hydrogen evolution: remarkably enhanced activity by dye sensitization [J].
Wang, Yabo ;
Hong, Jindui ;
Zhang, Wei ;
Xu, Rong .
CATALYSIS SCIENCE & TECHNOLOGY, 2013, 3 (07) :1703-1711
[35]   Visible light driven type II heterostructures and their enhanced photocatalysis properties: a review [J].
Wang, Yajun ;
Wang, Qisheng ;
Zhan, Xueying ;
Wang, Fengmei ;
Safdar, Muhammad ;
He, Jun .
NANOSCALE, 2013, 5 (18) :8326-8339
[36]   Polymeric Graphitic Carbon Nitride as a Heterogeneous Organocatalyst: From Photochemistry to Multipurpose Catalysis to Sustainable Chemistry [J].
Wang, Yong ;
Wang, Xinchen ;
Antonietti, Markus .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (01) :68-89
[37]   Graphene-Based Photocatalysts for Hydrogen Generation [J].
Xiang, Quanjun ;
Yu, Jiaguo .
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2013, 4 (05) :753-759
[38]   Graphene-based semiconductor photocatalysts [J].
Xiang, Quanjun ;
Yu, Jiaguo ;
Jaroniec, Mietek .
CHEMICAL SOCIETY REVIEWS, 2012, 41 (02) :782-796
[39]   Preparation and Enhanced Visible-Light Photocatalytic H2-Production Activity of Graphene/C3N4 Composites [J].
Xiang, Quanjun ;
Yu, Jiaguo ;
Jaroniec, Mietek .
JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (15) :7355-7363
[40]   Chemical exfoliation of graphitic carbon nitride for efficient heterogeneous photocatalysis [J].
Xu, Jing ;
Zhang, Liwu ;
Shi, Rui ;
Zhu, Yongfa .
JOURNAL OF MATERIALS CHEMISTRY A, 2013, 1 (46) :14766-14772