Anisotropic Electron-Phonon Coupling and Dynamical Nesting on the Graphene Sheets in Superconducting CaC6 using Angle-Resolved Photoemission Spectroscopy

被引:79
作者
Valla, T. [1 ]
Camacho, J. [1 ]
Pan, Z.-H. [2 ]
Fedorov, A. V. [2 ]
Walters, A. C. [3 ,4 ]
Howard, C. A. [3 ,4 ]
Ellerby, M. [3 ,4 ]
机构
[1] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA
[2] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA
[3] UCL, London Ctr Nanotechnol, London WC1E 6BT, England
[4] UCL, Dept Phys & Astron, London WC1E 6BT, England
基金
英国工程与自然科学研究理事会;
关键词
GRAPHITE; INTERCALATION; ENERGY; STATE;
D O I
10.1103/PhysRevLett.102.107007
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present the first angle-resolved photoemission studies of electronic structure in CaC6, a superconducting graphite intercalation compound with T-c=11.6 K. We find that, contrary to theoretical models, the electron-phonon coupling on the graphene-derived Fermi sheets with high-frequency graphene-derived phonons is surprisingly strong and anisotropic. The shape of the Fermi surface is found to favor a dynamical intervalley nesting via exchange of high-frequency phonons. Our results suggest that graphene sheets play a crucial role in superconductivity in graphite intercalation compounds.
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页数:4
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