Exact results for kinetics of catalytic reactions

被引:153
作者
Frachebourg, L [1 ]
Krapivsky, PL [1 ]
机构
[1] BOSTON UNIV, DEPT PHYS, BOSTON, MA 02215 USA
关键词
D O I
10.1103/PhysRevE.53.R3009
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
The kinetics of an irreversible catalytic reaction on a substrate of arbitrary dimension is examined. In the limit of infinitesimal reaction rate (reaction-controlled limit), we solve the dimer-dimer surface reaction model (or voter model) exactly in arbitrary dimension D. The density of reactive interfaces is found to exhibit a power-law decay for D<2 and a slow logarithmic decay in two dimensions. We discuss the relevance of these results for the monomer-monomer surface reaction model.
引用
收藏
页码:R3009 / R3012
页数:4
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