Controlling quantum transport through a single molecule

被引:245
作者
Cardamone, David M. [1 ]
Stafford, Charles A. [1 ]
Mazumdar, Sumit [1 ]
机构
[1] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA
基金
美国国家科学基金会;
关键词
D O I
10.1021/nl0608442
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We investigate multiterminal quantum transport through single monocyclic aromatic annulene molecules, and their derivatives, using the nonequilibrium Green function approach within the self-consistent Hartree-Fock approximation. We propose a new device concept, the quantum interference effect transistor, that exploits perfect destructive interference stemming from molecular symmetry and controls current flow by introducing decoherence and/or elastic scattering that break the symmetry. This approach overcomes the fundamental problems of power dissipation and environmental sensitivity that beset nanoscale device proposals.
引用
收藏
页码:2422 / 2426
页数:5
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