Targeted Synthesis of 2H-and 1T-Phase MoS2 Monolayers for Catalytic Hydrogen Evolution

被引：577

作者：

Chang, Kun ^{[1
]}

Hai, Xiao ^{[1
,2
]}

Pang, Hong ^{[1
,2
]}

Zhang, Huabin ^{[1
]}

Shi, Li ^{[1
,2
]}

Liu, Guigao ^{[1
,2
]}

Liu, Huimin ^{[1
]}

Zhao, Guixia ^{[1
]}

Li, Mu ^{[1
,2
]}

Ye, Jinhua ^{[1
,2
,3
,4
]}

机构：

[1] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton WPI MANA, 1-1Namiki, Tsukuba, Ibaraki 3050044, Japan

[2] Hokkaido Univ, Grad Sch Chem Sci & Engn, Sapporo, Hokkaido 0600814, Japan

[3] Tianjin Univ, Sch Mat Sci & Engn, TU NIMS Joint Res Ctr, 92 Weijin, Tianjin 300072, Peoples R China

[4] Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China

来源：

ADVANCED MATERIALS | 2016年 / 28卷 / 45期

基金：

美国国家科学基金会;

关键词：

ACTIVE EDGE SITES; ULTRATHIN NANOSHEETS; METAL; TRANSITION; INTERCALATION; EXFOLIATION; WATER; PHOTOLUMINESCENCE; PERFORMANCE;

D O I：

10.1002/adma.201603765

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Through a facile and effective strategy by employing lithium molten salts the controlled synthesis of 2H- and 1T-MoS2 monolayers with high-yield production is achieved. Both phases of MoS2 monolayers exhibit high stabilities. When used as a catalyst for hydrogen evolution, these phased MoS2 monolayers deliver respective advantages in the field of electro- and photo-catalytic hydrogen evolution.

引用

页码：10033 / 10041

页数：9

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