Laboratory and field investigations of particulate and carbon monoxide emissions from traditional and improved cookstoves

被引:248
作者
Roden, Christoph A. [1 ]
Bond, Tami C. [1 ]
Conway, Stuart [2 ]
Pinel, Anibal Benjamin Sorto [3 ]
MacCarty, Nordica [4 ]
Still, Dean [4 ]
机构
[1] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA
[2] Trees Water & People, Ft Collins, CO 80524 USA
[3] Colonia Country Club, AHDESA, Comayaguela, MDC, Honduras
[4] Aprovecho, Creswell, OR 97426 USA
基金
美国国家科学基金会;
关键词
Biofuel emissions; Cookstoves; Emission factors; Particulate matter; Elemental carbon; Organic carbon; FINE-PARTICLE EMISSIONS; OPTICAL-PROPERTIES; AEROSOL EMISSIONS; HOUSEHOLD STOVES; GREENHOUSE GASES; BLACK CARBON; WOOD; COMBUSTION; BIOMASS; DILUTION;
D O I
10.1016/j.atmosenv.2008.05.041
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
we implemented a program in which emission characterization is enabled through collaborations between academic, US and international non-govern mental entities that focus on evaluation, dissemination, and in-use testing, of improved cookstoves. This effort resulted in a study of field and laboratory emissions from traditional and improved biofuel cookstoves. We found that field measured particulate emissions of actual cooking average three times those measured during simulated cooking in the laboratory. Emission factors are highly dependent on the care and skill of the operator and the resulting combustion; these do not appear to be accurately reproduced in laboratory settings. The single scattering albedo (SSA) of the emissions was very low in both lab and field measurements, averaging about 0.3 for lab tests and around 0.5 for field tests, indicating that the primary particles are climate warming. Over the course of three summers in Honduras, we measured field emissions from traditional cookstoves, relatively new improved cookstoves, and "broken-in" improved cookstoves. We found that well-designed improved cookstoves can significantly reduce PM and CO emission factors below traditional cookstoves. For improved stoves, the presence of a chimney generally resulted in lower emission factors but left the SSA unaffected. Traditional cookstoves had an average PM emission factor of 8.2 g kg(-1) - significantly larger than previous studies. Particulate emission factors for improved cookstoves without and with chimneys averaged about 6.6 g kg(-1) and 4.5 g kg(-1), respectively. The elemental carbon (EC) fraction of PM varied significantly between individual tests, but averaged about 25% for each of the categories. (C) 2008 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1170 / 1181
页数:12
相关论文
共 38 条
[1]   THERMAL PERFORMANCE AND EMISSION CHARACTERISTICS OF UNVENTED BIOMASS-BURNING COOKSTOVES - A PROPOSED STANDARD METHOD FOR EVALUATION [J].
AHUJA, DR ;
JOSHI, V ;
SMITH, KR ;
VENKATARAMAN, C .
BIOMASS, 1987, 12 (04) :247-270
[2]  
Bailis R., 2007, Energy for Sustainable Development, VXI, P57, DOI DOI 10.1016/S0973-0826(08)60400-7
[3]  
BARNETT SG, 1981, 1981 INT C RES SOL F, P227
[4]   Trace gas and particle emissions from fires in large diameter and belowground biomass fuels [J].
Bertschi, I ;
Yokelson, RJ ;
Ward, DE ;
Babbitt, RE ;
Susott, RA ;
Goode, JG ;
Hao, WM .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D13)
[5]   Effects of selected parameters on performance and emission of biomass-fired cookstoves [J].
Bhattacharya, SC ;
Albina, DO ;
Khaing, AM .
BIOMASS & BIOENERGY, 2002, 23 (05) :387-395
[6]   Limitations in the enhancement of visible light absorption due to mixing state [J].
Bond, Tami C. ;
Habib, Gazala ;
Bergstrom, Robert W. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2006, 111 (D20)
[7]   A technology-based global inventory of black and organic carbon emissions from combustion [J].
Bond, TC ;
Streets, DG ;
Yarber, KF ;
Nelson, SM ;
Woo, JH ;
Klimont, Z .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D14) :D14203
[8]   STUDY OF WOOD STOVE PARTICULATE-EMISSIONS [J].
BUTCHER, SS ;
SORENSON, EM .
JOURNAL OF THE AIR POLLUTION CONTROL ASSOCIATION, 1979, 29 (07) :724-728
[9]   PARTICULATE EMISSION FACTORS FOR SMALL WOOD AND COAL STOVES [J].
BUTCHER, SS ;
ELLENBECKER, MJ .
JOURNAL OF THE AIR POLLUTION CONTROL ASSOCIATION, 1982, 32 (04) :380-384
[10]   Fuzzy relation equations (II): the branch-point-solutions and the categorized minimal solutions [J].
Chen, Li ;
Wang, Paul P. .
SOFT COMPUTING, 2007, 11 (01) :33-40