High loadings and source strengths of organic aerosols in China

被引:48
作者
Wang, Gehui
Kawamura, Kimitaka
Watanabe, Tomomi
Lee, Shuncheng
Ho, Kinfai
Cao, Junji
机构
[1] Hokkaido Univ, Inst Low Temp Sci, Kita Ku, Sapporo, Hokkaido 0600819, Japan
[2] Nanjing Univ, Sch Environm, State Key Lab Pollut Control & Resources Reuse, Nanjing 210008, Peoples R China
[3] Hong Kong Polytech Univ, Dept Civil & Struct Engn, Hong Kong, Hong Kong, Peoples R China
[4] Chinese Acad Sci, Inst Earth Environm, Xian, Peoples R China
关键词
D O I
10.1029/2006GL027624
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
Nation-wide studies of organic aerosols were conducted on a molecular level in 15 Chinese cities. The results showed strikingly high levels of organic compounds ( e. g., annual concentrations of polycyclic aromatic hydrocarbons, phthalates, sugars and diacids are 110, 370, 400 and 830 ng m(-3), respectively), especially in the mid-west region during winter ( up to 125 mu g m(-3) organic carbon). Fossil fuel combustion and/or biomass burning products are 3 - 30 times more abundant in winter than in summer. In contrast, significant quantity of phthalates ( 168 - 2200 ng m(-3)) was detected in summer. Concentrations of the pollutants are generally 1 - 3 orders of magnitude higher than those in developed countries. Their source strengths are characterized in winter by fossil fuel combustion, followed by secondary oxidation, plant wax emissions and biomass burning, whereas in summer by secondary oxidation, followed by fossil fuel combustion and plastic emissions.
引用
收藏
页数:4
相关论文
共 26 条
[1]   Global air quality and pollution [J].
Akimoto, H .
SCIENCE, 2003, 302 (5651) :1716-1719
[2]   China's burning ambition [J].
Aldhous, P .
NATURE, 2005, 435 (7046) :1152-1154
[3]   CONCENTRATIONS OF PARTICULATE AND GASEOUS POLYCYCLIC AROMATIC-HYDROCARBONS IN LONDON AIR FOLLOWING A REDUCTION IN THE LEAD CONTENT OF PETROL IN THE UNITED-KINGDOM [J].
BAEK, SO ;
GOLDSTONE, ME ;
KIRK, PWW ;
LESTER, JN ;
PERRY, R .
SCIENCE OF THE TOTAL ENVIRONMENT, 1992, 111 (2-3) :169-199
[4]   Emission factors for carbonaceous particles and polycyclic aromatic hydrocarbons from residential coal combustion in China [J].
Chen, YJ ;
Sheng, GY ;
Bi, XH ;
Feng, YL ;
Mai, BX ;
Fu, JM .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (06) :1861-1867
[5]   Construction of a 1° x 1° fossil fuel emission data set for carbonaceous aerosol and implementation and radiative impact in the ECHAM4 model [J].
Cooke, WF ;
Liousse, C ;
Cachier, H ;
Feichter, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D18) :22137-22162
[6]   Water-soluble organic compounds in biomass burning aerosols over Amazonia -: 1.: Characterization by NMR and GC-MS -: art. no. 8047 [J].
Graham, B ;
Mayol-Bracero, OL ;
Guyon, P ;
Roberts, GC ;
Decesari, S ;
Facchini, MC ;
Artaxo, P ;
Maenhaut, W ;
Köll, P ;
Andreae, MO .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D20) :LBA14-1
[7]   Seasonal variation of solvent extractable organic compounds in the aerosols in Qingdao, China [J].
Guo, ZG ;
Sheng, LF ;
Feng, JL ;
Fang, M .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (13) :1825-1834
[8]   Diurnal changes in the distribution of dicarboxylic acids, ketocarboxylic acids and dicarbonyls in the urban Tokyo atmosphere [J].
Kawamura, K ;
Yasui, O .
ATMOSPHERIC ENVIRONMENT, 2005, 39 (10) :1945-1960
[9]   Four years' observations of terrestrial lipid class compounds in marine aerosols from the western North Pacific [J].
Kawamura, K ;
Ishimura, Y ;
Yamazaki, K .
GLOBAL BIOGEOCHEMICAL CYCLES, 2003, 17 (01)
[10]   MOTOR EXHAUST EMISSIONS AS A PRIMARY SOURCE FOR DICARBOXYLIC-ACIDS IN LOS-ANGELES AMBIENT AIR [J].
KAWAMURA, K ;
KAPLAN, IR .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1987, 21 (01) :105-110