Hydrodynamics and propulsion mechanism of self-propelled catalytic micromotors: model and experiment

被引:78
作者
Li, Longqiu [1 ]
Wang, Jiyuan [1 ,2 ]
Li, Tianlong [1 ]
Song, Wenping [1 ]
Zhang, Guangyu [1 ]
机构
[1] Harbin Inst Technol, Harbin 150001, Peoples R China
[2] Heilongjiang Univ Sci & Technol, Harbin 150022, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
MICROJET ENGINES; BUBBLE FORMATION; MOLECULAR MOTOR; MICROENGINES; ORIFICE; LIQUID;
D O I
10.1039/c4sm01070a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070305 [高分子化学与物理];
摘要
The hydrodynamic behavior and propulsion mechanism of self-propelled micromotors are studied theoretically and experimentally. A hydrodynamic model to describe bubble growth and detachment is proposed to investigate the mechanism of a self-propelled conical tubular catalytic micromotor considering bubble geometric asymmetry and buoyancy force. The growth force caused by the growth of the bubble surface against the fluid is the driving force for micromotor motion. Also, the buoyancy force plays a primary role in bubble detachment. The effect of geometrical parameters on the micromotor velocity and drag force is presented. The bubble radius ratio is investigated for different micromotor radii to determine its hydrodynamic behavior during bubble ejection. The average micromotor velocity is found to be strongly dependent on the semi-cone angle, expelling frequency and bubble radius ratio. The semi-cone angle has a significant effect on the expelling frequency for conical tubular micromotors. The predicted results are compared to already existing experimental data for cylindrical micromotors (semi-cone angle delta = 0 degrees) and conical micromotors. A good agreement is found between the theoretical calculation and experimental results. This model provides a profound explanation for the propulsion mechanism of a catalytic micromotor and can be used to optimize the micromotor design for its biomedical and environmental applications.
引用
收藏
页码:7511 / 7518
页数:8
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