Giant intermolecular decay and fragmentation of clusters

被引:645
作者
Cederbaum, LS [1 ]
Zobeley, J [1 ]
Tarantelli, F [1 ]
机构
[1] UNIV PERUGIA,DIPARTIMENTO CHIM,I-06123 PERUGIA,ITALY
关键词
D O I
10.1103/PhysRevLett.79.4778
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
In sharp contrast to molecules, electronic states of clusters with an excited intermediate-shell electron can efficiently decay via an intermolecular Coulombic mechanism. Explicit examples are presented using large stale nb initio propagator calculations. The mechanism is illustrated and its generality is stressed.
引用
收藏
页码:4778 / 4781
页数:4
相关论文
共 34 条
[1]   SEMI-INTERNAL CORRELATION IN THE AUGER-ELECTRON SPECTRUM OF H2O [J].
AGREN, H ;
SIEGBAHN, H .
CHEMICAL PHYSICS LETTERS, 1980, 69 (03) :424-429
[2]  
Azaroff L.V., 1974, XRAY SPECTROSCOPY
[3]   CORRELATION-EFFECTS IN THE IONIZATION OF MOLECULES - BREAKDOWN OF THE MOLECULAR-ORBITAL PICTURE [J].
CEDERBAUM, LS ;
DOMCKE, W ;
SCHIRMER, J ;
VONNIESSEN, W .
ADVANCES IN CHEMICAL PHYSICS, 1986, 65 :115-159
[4]   ON DOUBLE VACANCIES IN THE CORE [J].
CEDERBAUM, LS ;
TARANTELLI, F ;
SGAMELLOTTI, A ;
SCHIRMER, J .
JOURNAL OF CHEMICAL PHYSICS, 1986, 85 (11) :6513-6523
[5]  
Chattarji D, 1976, THEORY AUGER TRANSIT
[6]   INTERCHANNEL COUPLING IN AUGER DECAY PROCESSES - CHARACTERIZATION OF NORMAL AND SATELLITE LINES IN THE AUGER-ELECTRON SPECTRUM OF THE LIF MOLECULE [J].
COLLE, R ;
SIMONUCCI, S .
PHYSICAL REVIEW A, 1990, 42 (07) :3913-3925
[7]   Ab initio block Lanczos calculation of the Auger spectra of SiF4: Strong two-hole localization effects and foreign imaging [J].
Gottfried, FO ;
Cederbaum, LS ;
Tarantelli, F .
PHYSICAL REVIEW A, 1996, 53 (04) :2118-2129
[8]   DOUBLE PHOTOIONIZATION OF CO2, OCS, C2H2, CF4, AND C6H6 STUDIED BY THRESHOLD PHOTOELECTRONS COINCIDENCE (TPESCO) SPECTROSCOPY [J].
HALL, RI ;
AVALDI, L ;
DAWBER, G ;
MCCONKEY, AG ;
MACDONALD, MA ;
KING, GC .
CHEMICAL PHYSICS, 1994, 187 (1-2) :125-135
[9]   The ab initio calculation of very many triply ionized states of molecular systems [J].
Handke, G ;
Tarantelli, F ;
Tarantelli, A ;
Cederbaum, LS .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 1995, 75 :109-115
[10]   UNIVERSAL GAUSSIAN-BASIS SETS FOR AN OPTIMUM REPRESENTATION OF RYDBERG AND CONTINUUM WAVEFUNCTIONS [J].
KAUFMANN, K ;
BAUMEISTER, W ;
JUNGEN, M .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1989, 22 (14) :2223-2240