Plasma methane conversion using dielectric-barrier discharges with zeolite A

被引:102
作者
Jiang, T
Li, Y
Liu, CJ [1 ]
Xu, GH
Eliasson, B
Xue, BZ
机构
[1] Tianjin Univ, State Key Lab Chem Technol C1, Tianjin 300072, Peoples R China
[2] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China
[3] ABB Corp Res Ltd, CH-5405 Baden, Switzerland
关键词
dielectric-barrier discharges; methane; carbon dioxide; zeolite A; syngas; hydrocarbons;
D O I
10.1016/S0920-5861(01)00497-7
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
Experimental investigation on plasma methane conversion in the presence of carbon dioxide using dielectric-barrier discharges (DBDs) has been conducted. Zeolite A has been applied to inhibit the formation of carbon black and plasma-polymerized film during such plasma methane conversion. A co-generation of syngas, light hydrocarbons and liquid fuels has been achieved. The conversions and selectivities are determined by the CH4/CO2 feed ratio, residence time and input power. Compared to the use of zeolite X within the DBDs, plasma methane conversion with zeolite A leads to a higher selectivity of light hydrocarbons (C-2-C-4). (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:229 / 235
页数:7
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