Magnetic resonance in the antiferromagnetic and normal state of NH3K3C60

被引:27
作者
Simon, F
Jánossy, A
Murányi, F
Fehér, T
Shimoda, H
Iwasa, Y
Forró, L
机构
[1] Tech Univ Budapest, Inst Phys, H-1521 Budapest, Hungary
[2] Japan Adv Inst Sci & Technol, Tatsunokuchi, Ishikawa 9231292, Japan
[3] Ecole Polytech Fed Lausanne, Lab Phys Solides Semicristallins, IGA Dept Phys, CH-1015 Lausanne, Switzerland
关键词
D O I
10.1103/PhysRevB.61.R3826
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report on the magnetic resonance of NH3K3C60 powders in the frequency range 9-225 GHz. The observation of an antiferromagnetic resonance below the phase transition at 40 K is evidence for an antiferromagnetically ordered ground state. In the normal state, above 40 K, the temperature dependence of the spin susceptibilty measured by electron-spin resonance agrees with previous static measurements and is too weak to be explained by interacting localized spins in an insulator. The magnetic-resonance linewidth has an unusual magnetic-field dependence which is large and temperature independent in the magnetically ordered state and decreases rapidly above the transition. These observations agree with the suggestion that NH3K3C60 is a metal in the normal state and undergoes a Mott-Hubbard metal to insulator transition at 40 K.
引用
收藏
页码:R3826 / R3829
页数:4
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