Exact results for the optical absorption of strongly correlated electrons in a half-filled Peierls-distorted chain

被引:37
作者
Gebhard, F
Bott, K
Scheidler, M
Thomas, P
Koch, SW
机构
[1] UNIV MARBURG,DEPT PHYS,D-35032 MARBURG,GERMANY
[2] UNIV MARBURG,CTR MAT SCI,D-35032 MARBURG,GERMANY
来源
PHILOSOPHICAL MAGAZINE B-PHYSICS OF CONDENSED MATTER STATISTICAL MECHANICS ELECTRONIC OPTICAL AND MAGNETIC PROPERTIES | 1997年 / 75卷 / 01期
关键词
D O I
10.1080/13642819708205701
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
In this, the second of three articles on the optical absorption of electrons in a half-filled Peierls-distorted chain, we present exact results for strongly correlated tight-binding electrons. In the limit of a strong on-site interaction U, we map the Hubbard model onto the Harris-Lange model which can be solved exactly in one dimension in terms of spinless fermions for the charge excitations. The exact solution allows for an interpretation of the charge dynamics in terms of parallel Hubbard bands with a free-electron dispersion of bandwidth W, separated by the Hubbard interaction U. The spin degrees of freedom enter the expressions for the optical absorption only via a momentum-dependent but static ground-state expectation value. The remaining spin problem can be traced out exactly since the eigenstates of the Harris-Lange model are spin degenerate. This corresponds to the Hubbard model at temperatures large compared with the spin exchange energy. Explicit results are given for the optical absorption in the presence of a lattice distortion delta and a nearest-neighbour interaction V. We find that the optical absorption for V = 0 is dominated by a peak at omega = U and broad but weak absorption bands for \omega - U\ less than or equal to W. For an appreciable nearest-neighbour interaction V > W/2, almost all the spectral weight is transferred to Simpson's exciton band which is eventually Peierls split.
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页码:13 / 46
页数:34
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