Third order nonlinear response of liquid water

被引:55
作者
Saito, S
Ohmine, I
机构
[1] Department of Chemistry, Faculty of Science, Nagoya University, Chikusa-ku, Nagoya 464-01, Furo-cho
关键词
D O I
10.1063/1.473538
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Third order nonlinear response of liquid water is investigated by using a classical molecular dynamics simulation. The calculated response function yields a marked agreement with the recent experimental results. The physical origins of the third order spectrum is analyzed in terms of the translational and the librational motions. Its temperature dependence and isotope effect are also analyzed. (C) 1997 American Institute of Physics.
引用
收藏
页码:4889 / 4893
页数:5
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