Initial Estimates of Mercury Emissions to the Atmosphere from Global Biomass Burning

被引:128
作者
Friedli, H. R. [1 ]
Arellano, A. F. [1 ]
Cinnirella, S. [2 ]
Pirrone, N. [2 ]
机构
[1] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[2] CNR, Inst Atmospher Pollut, Arcavacata Di Rende, Italy
基金
美国国家科学基金会;
关键词
BOREAL FOREST-FIRE; GASEOUS MERCURY; SOUTH-AFRICA; ECOSYSTEMS; TRANSPORT; POLLUTION; SMOKE;
D O I
10.1021/es802703g
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The average global annual mercury emission estimate from biomass burning (BMB) for 1997-2006 is 675 +/- 240 Mg/year. This is equivalent to 8% of all currently known anthropogenic and natural mercury emissions. By season, the largest global emissions occur in August and September, the lowest during northern winters. The interannual variability is large and region-specific, and responds to drought conditions. During this particular time period, the largest mercury emissions are from tropical and boreal Asia, followed by Africa and South America. They do not coincide with the largest carbon biomass burning emissions, which originate from Africa. Frequently burning grasslands in Africa and Australia, and agricultural waste burning globally, contribute relatively little to the mercury budget. The released mercury from BMB is eventually deposited locally and globally and contributes to the formation of toxic bioaccumulating methyl mercury. Furthermore, increasing temperature in boreal regions, where the largest soil mercury pools reside, is expected to exacerbate mercury emission because of more frequent, larger, and more intense fires.
引用
收藏
页码:3507 / 3513
页数:7
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