Analysis and interpretation of the continuous hourly monitoring data for 26 C2-C8 hydrocarbons at 12 United Kingdom sites during 1996

被引:162
作者
Derwent, RG
Davies, TJ
Delaney, M
Dollard, GJ [2 ]
Field, RA
Dumitrean, P
Nason, PD
Jones, BMR
Pepler, SA
机构
[1] Meteorol Off, Div Climate Res, Bracknell RB12 2SZ, Berks, England
[2] AEA Technol Environm, NETCEN, Culham, Oxon, England
关键词
VOCs; automatic monitoring; motor vehicle emissions; industrial sources; urban VOC concentrations;
D O I
10.1016/S1352-2310(99)00203-4
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A fully automatic network with 11 urban background and one rural site has been set up and operated successfully in the UK to measure, continuously, hourly concentrations of 26 C-2-C-8 hydrocarbons; the measurements collected form one of the largest data sets of urban hydrocarbon air quality data available anywhere in Europe. The hourly data have been analysed on a site-by-site and hydrocarbon-by-hydrocarbon basis by constructing scatter plots against benzene. From: these scatter plots a number of important sources of hydrocarbon emissions have clearly been identified including: motor vehicle exhaust and evaporative emissions, natural gas leakage, petrol station forecourt evaporative emissions and industrial sources. Overall, urban background hydrocarbon air quality-is heavily influenced by motor vehicles and the general pattern of relative concentrations has been accurately defined for the United Kingdom as ratios relative to benzene. Comparisons of these concentrations are made with data for other major cities and with European regional data. (C) 1999 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:297 / 312
页数:16
相关论文
共 24 条
[1]  
[Anonymous], 1987, WHO REG PUBL EUR SER
[2]  
*ASS OCT, 1978, OCT GROUP GAS SURV
[3]   GAS-PHASE TROPOSPHERIC CHEMISTRY OF ORGANIC-COMPOUNDS - A REVIEW [J].
ATKINSON, R .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1990, 24 (01) :1-41
[4]   SEASONAL-VARIATION OF ATMOSPHERIC NONMETHANE HYDROCARBONS ON THE WESTERN COAST OF BRITTANY, FRANCE [J].
BOUDRIES, H ;
TOUPANCE, G ;
DUTOT, AL .
ATMOSPHERIC ENVIRONMENT, 1994, 28 (06) :1095-1112
[5]   THE OCCURRENCE OF CHLORINATED AND OTHER ORGANIC TRACE COMPOUNDS IN URBAN AIR [J].
BRUCKMANN, P ;
KERSTEN, W ;
FUNCKE, W ;
BALFANZ, E ;
KONIG, J ;
THEISEN, J ;
BALL, M ;
PAPKE, O .
CHEMOSPHERE, 1988, 17 (12) :2363-2380
[6]  
Derwent R.G., 1995, Issues in Environ. Sci.Technol. v, V4, P1
[7]   ANALYSIS AND INTERPRETATION OF AIR-QUALITY DATA FROM AN URBAN ROADSIDE LOCATION IN CENTRAL LONDON OVER THE PERIOD FROM JULY 1991 TO JULY 1992 [J].
DERWENT, RG ;
MIDDLETON, DR ;
FIELD, RA ;
GOLDSTONE, ME ;
LESTER, JN ;
PERRY, R .
ATMOSPHERIC ENVIRONMENT, 1995, 29 (08) :923-946
[8]  
DOLLARD GJ, 1995, ISSUES ENV SCI TECHN, V4, P37
[9]   Non-methane exhaust composition in the Sydney Harbour Tunnel: A focus on benzene and 1,3-butadiene [J].
Duffy, BL ;
Nelson, PF .
ATMOSPHERIC ENVIRONMENT, 1996, 30 (15) :2759-2768
[10]  
*EEA, 1995, COR SUMM TABL