The photophysics of organic semiconducting nanospheres: a comprehensive study

被引:16
作者
Piok, T
Gadermaier, C
Wenzl, FP
Patil, S
Montenegro, R
Landfester, K
Lanzani, G
Cerullo, G
Scherf, U
List, EJW
机构
[1] Graz Univ Technol, Inst Solid State Phys, Christian Doppler Lab Adv Funct Mat, A-8010 Graz, Austria
[2] Inst Nanostruct Mat & Photon, A-8160 Weiz, Austria
[3] Graz Univ Technol, Inst Solid State Phys, A-8010 Graz, Austria
[4] Berg Univ Wuppertal, D-42097 Wuppertal, Germany
[5] Univ Ulm, D-89069 Ulm, Germany
[6] Natl Lab Ultrafast & Ultraintense Opt Sci, I-20133 Milan, Italy
[7] Politecn Milan, Dipartimento Fis, INFM, I-20133 Milan, Italy
关键词
D O I
10.1016/j.cplett.2004.03.018
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The steady-state and non equilibrium photoexcitation dynamics of semiconducting polymer nanospheres is studied in detail and compared to a regular bulk film of the same polymer (methyl-substituted ladder-type poly(para)phenylene). It is found that the major optical properties of the polymer are left unaltered by this innovative material processing approach. However there is a clear influence of the film nanostructure on the generation, migration and recombination behavior of the involved photoexcited species. (C) 2004 Elsevier B.V. All rights reserved.
引用
收藏
页码:7 / 13
页数:7
相关论文
共 30 条
[1]   PHOTOINDUCED ABSORPTION OF POLYMER-SOLUTIONS [J].
BOTTA, C ;
LUZZATI, S ;
TUBINO, R ;
BRADLEY, DDC ;
FRIEND, RH .
PHYSICAL REVIEW B, 1993, 48 (20) :14809-14817
[2]   Dispersive dynamics of photoexcitations in conjugated polymers measured by photomodulation spectroscopy [J].
Epshtein, O ;
Nakhmanovich, G ;
Eichen, Y ;
Ehrenfreund, E .
PHYSICAL REVIEW B, 2001, 63 (12)
[3]   Electroluminescence in conjugated polymers [J].
Friend, RH ;
Gymer, RW ;
Holmes, AB ;
Burroughes, JH ;
Marks, RN ;
Taliani, C ;
Bradley, DDC ;
Dos Santos, DA ;
Brédas, JL ;
Lögdlund, M ;
Salaneck, WR .
NATURE, 1999, 397 (6715) :121-128
[4]   Ultrafast photoexcitation dynamics in a ladder-type oligophenyl -: art. no. 125203 [J].
Gadermaier, C ;
Cerullo, G ;
Zavelani-Rossi, M ;
Sansone, G ;
Lanzani, G ;
Zojer, E ;
Pogantsch, A ;
Beljonne, D ;
Shuai, Z ;
Brédas, JL ;
Scherf, U ;
Leising, G .
PHYSICAL REVIEW B, 2002, 66 (12) :1252031-1252037
[5]   Photophysics of conjugated polymers: the contribution of ultrafast spectroscopy [J].
Gadermaier, C ;
Lanzani, G .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2002, 14 (42) :9785-9802
[6]   ALL-POLYMER FIELD-EFFECT TRANSISTOR REALIZED BY PRINTING TECHNIQUES [J].
GARNIER, F ;
HAJLAOUI, R ;
YASSAR, A ;
SRIVASTAVA, P .
SCIENCE, 1994, 265 (5179) :1684-1686
[7]   Femtosecond relaxation of photoexcitations in a poly(para-phenylene)-type ladder polymer [J].
Graupner, W ;
Leising, G ;
Lanzani, G ;
Nisoli, M ;
DeSilvestri, S ;
Scherf, U .
PHYSICAL REVIEW LETTERS, 1996, 76 (05) :847-850
[8]   All-polymer optoelectronic devices [J].
Ho, PKH ;
Thomas, DS ;
Friend, RH ;
Tessler, N .
SCIENCE, 1999, 285 (5425) :233-236
[9]   TRIPLET-STATE PHOTOEXCITATIONS OF OLIGOTHIOPHENE FILMS AND SOLUTIONS [J].
JANSSEN, RAJ ;
SMILOWITZ, L ;
SARICIFTCI, NS ;
MOSES, D .
JOURNAL OF CHEMICAL PHYSICS, 1994, 101 (03) :1787-1798
[10]  
Landfester K, 2001, ADV MATER, V13, P765, DOI 10.1002/1521-4095(200105)13:10<765::AID-ADMA765>3.0.CO