Measurements of ice water content in tropopause region arctic cirrus during the SAGE III Ozone Loss and Validation Experiment (SOLVE)

被引:21
作者
Hallar, AG
Avallone, LM
Herman, RL
Anderson, BE
Heymsfield, AJ
机构
[1] Univ Colorado, Program Atmospher & Ocean Sci, Boulder, CO 80309 USA
[2] NASA, Langley Res Ctr, Hampton, VA 23681 USA
[3] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA
[4] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
关键词
ice water content; cirrus; heterogeneous chemistry;
D O I
10.1029/2003JD004348
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
[1] A new instrument, the closed-path laser hygrometer (CLH), was flown on the NASA DC-8 aircraft during the Stratospheric Aerosol and Gas Experiment (SAGE) III Ozone Loss and Validation Experiment ( SOLVE) campaign in 1999 - 2000 to measure condensed-phase water. The ice water content (IWC) of Arctic cirrus was determined from in situ measurements of condensed- and gas-phase water. The IWC values obtained from the CLH observations are compared to those determined by integrating particle size distributions measured by a Forward Scattering Spectrometer Probe (FSSP) also flown on the DC-8. The considerably greater IWC seen by the CLH implies the presence of particles with diameters greater than the FSSP's upper limit of 20 mm. The evidence for and implications of the presence of large ice crystals in Arctic cirrus is discussed.
引用
收藏
页码:D172031 / 9
页数:9
相关论文
共 64 条
[1]   Interaction of HNO3 with water-ice surfaces at temperatures of the free troposphere [J].
Abbatt, JPD .
GEOPHYSICAL RESEARCH LETTERS, 1997, 24 (12) :1479-1482
[2]   INTERPRETATION OF MEASUREMENTS MADE BY THE FORWARD SCATTERING SPECTROMETER PROBE (FSSP-300) DURING THE AIRBORNE ARCTIC STRATOSPHERIC EXPEDITION [J].
BAUMGARDNER, D ;
DYE, JE ;
GANDRUD, BW ;
KNOLLENBERG, RG .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1992, 97 (D8) :8035-8046
[3]  
BELYAEV SP, 1972, AEROSOL SCIENCE, V3, P127
[4]  
BOOKER DR, 1982, C CLOUD PHYS AM MET
[5]   The potential of cirrus clouds for heterogeneous chlorine activation [J].
Borrmann, S ;
Solomon, S ;
Dye, JE ;
Luo, BP .
GEOPHYSICAL RESEARCH LETTERS, 1996, 23 (16) :2133-2136
[6]   Chemical ozone loss in the tropopause region on subvisible ice clouds, calculated with a chemistry-transport model [J].
Bregman, B ;
Wang, PH ;
Lelieveld, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D3)
[7]   The impact of temperature errors on perceived humidity supersaturation [J].
Buehler, SA ;
Courcoux, N .
GEOPHYSICAL RESEARCH LETTERS, 2003, 30 (14) :ASC11-1
[8]  
DOWLING DR, 1990, J APPL METEOROL, V29, P970, DOI 10.1175/1520-0450(1990)029<0970:ASOTPP>2.0.CO
[9]  
2
[10]   INSITU MEASUREMENTS OF TOTAL REACTIVE NITROGEN, TOTAL WATER, AND AEROSOL IN A POLAR STRATOSPHERIC CLOUD IN THE ANTARCTIC [J].
FAHEY, DW ;
KELLY, KK ;
FERRY, GV ;
POOLE, LR ;
WILSON, JC ;
MURPHY, DM ;
LOEWENSTEIN, M ;
CHAN, KR .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1989, 94 (D9) :11299-11315