Isoprene and monoterpene emissions from an Inner Mongolia grassland

被引:43
作者
Bai, Jianhui
Baker, Bradly
Liang, Baosheng
Greenberg, James
Guenther, Alex
机构
[1] Natl Ctr Atmospher Res, Boulder, CO 80305 USA
[2] Chinese Acad Sci, Inst Atmospher Phys, LAGEO, Beijing 100029, Peoples R China
[3] Calif State Univ Sacramento, Dept Chem, Sacramento, CA 95819 USA
[4] Peking Univ, Environm Coll, Beijing 100871, Peoples R China
基金
美国国家科学基金会;
关键词
biogenic emissions inventory; Carex; China; volatile organic compounds (VOCs);
D O I
10.1016/j.atmosenv.2006.05.019
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Terpenoid emissions were measured at a grassland site in Inner Mongolia, China during four campaigns over a 2-year period. Emissions were strongly correlated with light and temperature and the variations could be simulated using a canopy emission model. Substantial seasonal and interannual variations in isoprene emissions were also observed. Area averaged isoprene emissions normalized to standard above-canopy temperature and light conditions (30 degrees C and 1500 mu mol m(-2) s(-1)) ranged from about 50 to 500 mu g m(-2) h(-1). These rates are more than an order of magnitude higher than those previously reported for temperate grasslands but are lower than emission rates observed from ground cover vegetation at higher latitudes. Isoprene emissions from this Inner Mongolia grassland may be dominated by emissions from sedges, e.g. Carex appendiculata. Total monoterpene emissions normalized to a standard temperature of 30 degrees C were only about 3 mu g m(-2) h(-1) and consisted primarily of carene and limonene with smaller contributions of a-pinene and beta-pinene. A model sensitivity study showed that grass and other herbaceous ground cover can contribute > 10% of the total isoprene emission from certain regions, such as Inner Mongolia, but are < 4% on a global annual scale. (c) 2006 Elsevier Ltd. All rights reserved.
引用
收藏
页码:5753 / 5758
页数:6
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