Dielectric spectra in charge ordering state of Pr1-xCaxMnO3

被引:29
作者
Yamada, S [1 ]
Arima, T [1 ]
Takita, K [1 ]
机构
[1] Univ Tsukuba, Inst Mat Sci, Tsukuba, Ibaraki 3058573, Japan
关键词
dielectric spectra; manganese oxide; charge ordering; transport properties; colossal magnetoresistance;
D O I
10.1143/JPSJ.68.3701
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We measured dielectric spectra in the charge ordering state of Pr1-xCaxMnO3 (0.30 less than or equal to x less than or equal to 0.50); for frequencies of 100 Hz similar to 15 MHz. Observed dielectric spectra were analyzed using the Debye model. The effective number of electrons (n/m) is nearly temperature independent. Dissipation, gamma, drastically increases with cooling. Temperature dependence is almost the same as resistivity curve. This indicates that the hopping of polarons dominate both dc- and ac-electrical transport in the charge ordering phase. Based on the small-polaron-hopping model, x-dependent activation energy is estimated, which reaches a maximum at x similar or equal to 0.33. The gamma-value decreases in magnetic fields, hut does not scale with magnetization.
引用
收藏
页码:3701 / 3707
页数:7
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