Approaches to wave packet imaging using femtosecond ionization spectroscopy

被引：8

作者：

Gräfe, S

Scheidel, D

Engel, V

Henriksen, NE

Moller, KB

机构：

[1] Univ Wurzburg, Inst Chem Phys, D-97074 Wurzburg, Germany

[2] Tech Univ Denmark, Dept Chem, DK-2800 Lyngby, Denmark

来源：

JOURNAL OF PHYSICAL CHEMISTRY A | 2004年 / 108卷 / 41期

关键词：

D O I：

10.1021/jp040230q

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Different methods to obtain information about the probability densities of vibrational wave packets in diatomic molecule are compared. More explicitly, we consider pump-probe ionization processes. Time-resolved photoelectron spectra and total ion yields as well as fragment ion distributions are calculated, and these different quantities are employed to reconstruct radial densities. It is shown that pump-probe ionization experiments are well suited for the mapping of vibrational wave packets.

引用

收藏

页码：8954 / 8960

页数：7

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