Coupling of ferroelectric and antiferromagnetic order parameters in hexagonal RMnO3

被引:6
作者
Lottermoser, T [1 ]
Fiebig, M [1 ]
Fröhlich, D [1 ]
Kallenbach, S [1 ]
Maat, M [1 ]
机构
[1] Univ Dortmund, Inst Phys, D-44221 Dortmund, Germany
来源
APPLIED PHYSICS B-LASERS AND OPTICS | 2002年 / 74卷 / 7-8期
关键词
D O I
10.1007/s003400200836
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Second-harmonic generation (SHG) is used as a probe for the coexisting ferroelectric and antiferromagnetic orders in hexagonal RMnO3. SH contributions coupling to the electric and/or magnetic order parameters are identified on the basis of their spectral dependence and the symmetries of the corresponding order parameters. The SH signals from the ferroelectric and antiferromagnetic orders were employed to image the electric and magnetic domain structures separately. The transformation properties of electric and magnetic domains are discussed with respect to the transformation properties of the corresponding order parameters. An investigation of the mutual coupling between the coexisting electric and magnetic orders reveals apparently independent domain structures, which contradicts the symmetry and transformation properties of electric-dipole-induced SHG in this ferroelectromagnetic group of compounds. Apart from higher-order multipole contributions to SHG, interface contributions from clamped electric and magnetic domains can solve the contradiction.
引用
收藏
页码:759 / 764
页数:6
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