Study of biodegradation processes along the Carnaubais trend, Potiguar Basin (Brazil) - Part 1

被引:23
作者
Behar, F.
Penteado, H. L. de Barros
Lorant, F.
Budzinski, H.
机构
[1] IFP Energies Nouvelles, Direct Geol Geochim, F-92506 Rueil Malmaison, France
[2] Petrobras R&D Ctr, Cenpes PDEXP, GEOQ, Rio De Janeiro, Brazil
[3] Univ Bordeaux 1, Lab Phys & Toxicochim Syst Nat, CNRS, URA 348, F-33400 Talence, France
关键词
D O I
10.1016/j.orggeochem.2006.05.009
中图分类号
P3 [地球物理学]; P59 [地球化学];
学科分类号
0708 [地球物理学]; 070902 [地球化学];
摘要
The aim of this study is to estimate hydrocarbon losses in natural reservoirs due to biodegradation processes. A series of 12 non-biodegraded and biodegraded oils were selected in the Potiguar Basin (Brazil). Most biodegraded reservoir oils are located in the southwestern part of the basin (onshore), within the Cretaceous sandstones of the Agu units that occur at shallow depths (< 1000 m). Deeper reservoirs, containing non-biodegraded but mature oils, are located in the northeastern area of the basin. Based on the chemical alteration of the saturates and aromatics observed in biodegraded oils, tentative estimates of absolute losses were calculated for the light hydrocarbons (saturates and aromatics) and for the heavy fractions such as C14+ linear and cyclo-alkanes and C14+ aromatics. Together with the estimation of losses on global classes, molecular studies clearly show that biodegradation scales based on saturated and aromatic biomarkers can be used as such but do not reflect the loss percentage by biodegradation on global classes. (c) 2006 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1042 / 1051
页数:10
相关论文
共 25 条
[1]
Araripe P. T., 1994, Boletim de Geociencias Da Petrobras, V8, P127
[2]
Methane generation from oil cracking: Kinetics of 9-methylphenanthrene cracking and comparison with other pure compounds and oil fractions [J].
Behar, F ;
Budzinski, H ;
Vandenbroucke, M ;
Tang, Y .
ENERGY & FUELS, 1999, 13 (02) :471-481
[3]
Bertani R.T., 1990, ORIGEM EVOLUCAAAO BA, P291
[4]
BLANCHET D, 2005, MICROBIOLOGIE PETROL, V2, P629
[5]
BUDZINSKI H, 1992, THESIS U BORDEAUX FR
[6]
Connan J., 1984, ADV PETROLEUM GEOCHE, V1, P299, DOI [10.1016/B978-0-12-032001-1.50011-0, DOI 10.1016/B978-0-12-032001-1.50011-0]
[7]
GARRIGUES P, 1983, ORG GEOCHEM, V5, P53
[8]
HOOD A, 1959, ADV MASS SPECTROM, P175
[9]
Johns RB., 1986, BIOL MARKERS SEDIMEN
[10]
The controls on the composition of biodegraded oils in the deep subsurface - part 1: biodegradation rates in petroleum reservoirs [J].
Larter, S ;
Wilhelins, A ;
Head, I ;
Koopmans, M ;
Aplin, A ;
Di Primio, R ;
Zwach, C ;
Erdmann, M ;
Telnaes, N .
ORGANIC GEOCHEMISTRY, 2003, 34 (04) :601-613