Selective catalytic reduction of N2O by C3H6 over Fe-MFI

被引:39
作者
Pophal, C
Yogo, T
Tanabe, K
Segawa, K
机构
[1] SOPHIA UNIV,FAC SCI & TECHNOL,DEPT CHEM,CHIYODA KU,TOKYO 102,JAPAN
[2] TH DARMSTADT,FACHBEREICH MAT WISSENSCH,D-64287 DARMSTADT,GERMANY
关键词
nitrous oxide; propene; selective reduction; Fe-MFI; Cu-MFI;
D O I
10.1023/A:1018914100881
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The catalytic activities of Fe-MFI (88% exchange) and Cu-MFI (122% exchange) zeolite catalysts for the decomposition and mainly the selective reduction of nitrous oxide by propene have been studied in the temperature range from 523 to 773 K. In the presence of oxygen and water vapor, both materials reveal strong retardation of their activity. When propene is added as reductant, Fe-MFI showed very high activity even in the low-temperature region and at low propene concentrations, whereas Cu-MFI is strongly deactivated.
引用
收藏
页码:271 / 274
页数:4
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