Particulate and dissolved 210Pb activities in the shelf and slope regions of the Gulf of Mexico waters

被引:41
作者
Baskaran, M [1 ]
Santschi, PH
机构
[1] Wayne State Univ, Dept Geol, Detroit, MI 49202 USA
[2] Texas A&M Univ, Dept Marine Sci, Galveston, TX 77551 USA
基金
美国国家科学基金会;
关键词
boundary scavenging; warm-core ring; dissolved and particulate Pb-210; residence time of Pb-210; scavenging index; distribution coefficicnts;
D O I
10.1016/S0278-4343(02)00017-1
中图分类号
P7 [海洋学];
学科分类号
0707 ;
摘要
Concentration profiles of dissolved and particulate Pb-210 were measured on horizontal transects of the continental shelf and slope regions of the Gulf of Mexico. Vertical profiles in the slope station in the presence and absence of warm-core ring enable us to evaluate the differences in the scavenging intensity of Pb-210. A comparison of the rate of production of Pb-210 in the overlying water column to that of its mean annual flux calculated from the sediment inventory allows us to get a better insight in to the lateral transport and deposition of Pb-210 to the slope sediments over a < 100 year time scale. Our results indicate that there is no general increase of dissolved or particulate Pb-210 concentration with depth. The scavenging residence time of Pb-210 for the entire 1500-m water column varied between 0.06 and 4.7 years. There was a strong correlation between the inventory of total (dissolved + particulate) Pb-210 and depth of the water column. The ratio of measured sediment inventory (F) of Pb-210 to its production (P) in the overlying water column varied between 0.69 and 1.63, suggesting that, at time, lateral inputs from boundary scavenging in a few sites are dominant, while in other places, vertical scavenging is the primary mechanism of transport for Pb-210. (C) 2002 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:1493 / 1510
页数:18
相关论文
共 44 条
[1]   ANOMALOUS BOUNDARY SCAVENGING IN THE MIDDLE ATLANTIC BIGHT - EVIDENCE FROM TH-230, PA-231, BE-1O AND PB-210 [J].
ANDERSON, RF ;
FLEISHER, MQ ;
BISCAYE, PE ;
KUMAR, N ;
DITRICH, B ;
KUBIK, P ;
SUTER, M .
DEEP-SEA RESEARCH PART II-TOPICAL STUDIES IN OCEANOGRAPHY, 1994, 41 (2-3) :537-561
[2]   MIXING OF PARTICLES AND ORGANIC-CONSTITUENTS IN SEDIMENTS FROM THE CONTINENTAL-SHELF AND SLOPE OFF CAPE-COD - SEEP-I RESULTS [J].
ANDERSON, RF ;
BOPP, RF ;
BUESSELER, KO ;
BISCAYE, PE .
CONTINENTAL SHELF RESEARCH, 1988, 8 (5-7) :925-946
[3]   PB-210-RA-226 AND PO-210-PB-210 DISEQUILIBRIA IN SEAWATER AND SUSPENDED PARTICULATE MATTER [J].
BACON, MP ;
SPENCER, DW ;
BREWER, PG .
EARTH AND PLANETARY SCIENCE LETTERS, 1976, 32 (02) :277-296
[4]   PB-210 BALANCE AND IMPLICATIONS FOR PARTICLE-TRANSPORT ON THE CONTINENTAL-SHELF, US MIDDLE ATLANTIC BIGHT [J].
BACON, MP ;
BELASTOCK, RA ;
BOTHNER, MH .
DEEP-SEA RESEARCH PART II-TOPICAL STUDIES IN OCEANOGRAPHY, 1994, 41 (2-3) :511-535
[5]   PB-210 AND PO-210 IN OCEAN WATER PROFILES OF THE CONTINENTAL-SHELF AND SLOPE SOUTH OF NEW-ENGLAND [J].
BACON, MP ;
BELASTOCK, RA ;
TECOTZKY, M ;
TUREKIAN, KK ;
SPENCER, DW .
CONTINENTAL SHELF RESEARCH, 1988, 8 (5-7) :841-853
[6]   A METHOD FOR RAPID INSITU EXTRACTION AND LABORATORY DETERMINATION OF TH, PB, AND RA ISOTOPES FROM LARGE VOLUMES OF SEAWATER [J].
BASKARAN, M ;
MURPHY, DJ ;
SANTSCHI, PH ;
ORR, JC ;
SCHINK, DR .
DEEP-SEA RESEARCH PART I-OCEANOGRAPHIC RESEARCH PAPERS, 1993, 40 (04) :849-865
[7]   PB-210-DERIVED CHRONOLOGY AND THE FLUXES OF PB-210 AND CS-137 ISOTOPES INTO CONTINENTAL-SHELF SEDIMENTS, EAST-CHUKCHI-SEA, ALASKAN ARCTIC [J].
BASKARAN, M ;
NAIDU, AS .
GEOCHIMICA ET COSMOCHIMICA ACTA, 1995, 59 (21) :4435-4448
[8]   ATMOSPHERIC DEPOSITIONAL FLUXES OF BE-7 AND PB-210 AT GALVESTON AND COLLEGE-STATION, TEXAS [J].
BASKARAN, M ;
COLEMAN, CH ;
SANTSCHI, PH .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1993, 98 (D11) :20555-20571
[9]   THE ROLE OF PARTICLES AND COLLOIDS IN THE TRANSPORT OF RADIONUCLIDES IN COASTAL ENVIRONMENTS OF TEXAS [J].
BASKARAN, M ;
SANTSCHI, PH .
MARINE CHEMISTRY, 1993, 43 (1-4) :95-114
[10]   Th-234:U-238 disequilibria in the Gulf of Mexico: The importance of organic matter and particle concentration [J].
Baskaran, M ;
Santschi, PH ;
Guo, LD ;
Bianchi, TS ;
Lambert, C .
CONTINENTAL SHELF RESEARCH, 1996, 16 (03) :353-380