Three-dimensional thermo-fluid electrochemical modeling of planar SOFC stacks

被引:271
作者
Recknagle, KP [1 ]
Williford, RE [1 ]
Chick, LA [1 ]
Rector, DR [1 ]
Khaleel, MA [1 ]
机构
[1] Pacific NW Natl Lab, Richland, WA 99352 USA
关键词
solid oxide fuel cell; three-dimensional model; fuel utilization; current and temperature distribution;
D O I
10.1016/S0378-7753(02)00487-1
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A simulation tool for modeling planar solid oxide fuel cells is demonstrated. The tool combines the versatility of a commercial computational fluid dynamics simulation code with a validated electrochemistry calculation method. Its function is to predict the flow and distribution of anode and cathode gases, temperature and current distributions, and fuel utilization. A three-dimensional model geometry, including internal manifolds, was created to simulate a generic, cross-flow stack design. Similar three-dimensional geometries were created for simulation of co-flow, and counterflow stack designs. Cyclic boundary conditions were imposed at the top and bottom of the model domains, while the lateral walls were assumed adiabatic. The three cases show that, for a given average cell temperature, similar fuel utilizations can result irrespective of the flow configuration. Temperature distributions however, which largely determine thermal, stresses during operation, are dependent on the chosen design geometry/flow configuration. The co-flow case had the most uniform temperature distribution and the smallest thermal gradients, thus offers thermo-structural advantages over the other flow cases. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:109 / 114
页数:6
相关论文
共 8 条
[1]  
CHICK LA, 2000, 2000 FUEL CELL SEM, P619
[2]  
*COMP DYN LTD, 1998, STAR CD VERS 3 05 MA
[3]   Performance analysis of planar-type unit SOFC considering current and temperature distributions [J].
Iwata, M ;
Hikosaka, T ;
Morita, M ;
Iwanari, T ;
Ito, K ;
Onda, K ;
Esaki, Y ;
Sakaki, Y ;
Nagata, S .
SOLID STATE IONICS, 2000, 132 (3-4) :297-308
[4]  
KEEGAN K, 2002, C 2002 P SOC AUT ENG
[5]   The reversed flow operation of a crossflow solid oxide fuel cell monolith [J].
Neophytides, SG .
CHEMICAL ENGINEERING SCIENCE, 1999, 54 (20) :4603-4613
[6]  
Yakabe H, 1999, ELEC SOC S, V99, P1087
[7]   3-D model calculation for planar SOFC [J].
Yakabe, H ;
Ogiwara, T ;
Hishinuma, M ;
Yasuda, I .
JOURNAL OF POWER SOURCES, 2001, 102 (1-2) :144-154
[8]   Evaluation and modeling of performance of anode-supported solid oxide fuel cell [J].
Yakabe, H ;
Hishinuma, M ;
Uratani, M ;
Matsuzaki, Y ;
Yasuda, I .
JOURNAL OF POWER SOURCES, 2000, 86 (1-2) :423-431