Model catalysts: reductionism for understanding

被引:37
作者
Boudart, M [1 ]
机构
[1] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA
关键词
model catalysts; information; understanding;
D O I
10.1023/A:1009080821550
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
A model heterogeneous catalyst is synthesized for the purpose of understanding how it works. The model is inspired by a real catalyst. The latter is made simpler with a known structure and texture, with identifiable and countable sites. The goal is to approach the ideal molecular catalyst with identical and non-interacting active sites, i.e., a single site catalyst. Five examples of model catalysts are discussed with the understanding gained from their study.
引用
收藏
页码:147 / 149
页数:3
相关论文
共 17 条
[2]   SURFACE, CATALYTIC AND MAGNETIC-PROPERTIES OF SMALL IRON PARTICLES .1. PREPARATION AND CHARACTERIZATION OF SAMPLES [J].
BOUDART, M ;
DELBOUILLE, A ;
DUMESIC, JA ;
KHAMMOUMA, S ;
TOPSOE, H .
JOURNAL OF CATALYSIS, 1975, 37 (03) :486-502
[3]   SURFACE-STRUCTURE OF IRON CATALYSTS FOR AMMONIA-SYNTHESIS [J].
BOUDART, M ;
LOFFLER, DG .
JOURNAL OF PHYSICAL CHEMISTRY, 1984, 88 (23) :5763-5763
[4]   PAULINGS THEORY OF METALS IN CATALYSIS [J].
BOUDART, M .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1950, 72 (02) :1040-1040
[5]   The relevance in practice of data obtained on heterogeneous model catalysts [J].
Boudart, M .
ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS, 1996, 197 :21-35
[6]   Heterogeneous molecular catalysis: Oxymoron or reality? [J].
Boudart, M .
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 1997, 120 (1-3) :271-280
[7]  
DUKE CB, 1994, SURFACE SCI 1 30 YEA, P1054
[8]   SURFACE, CATALYTIC AND MAGNETIC-PROPERTIES OF SMALL IRON PARTICLES .3. NITROGEN INDUCED SURFACE RECONSTRUCTION [J].
DUMESIC, JA ;
TOPSOE, H ;
BOUDART, M .
JOURNAL OF CATALYSIS, 1975, 37 (03) :513-522
[9]  
HAAG WO, 1994, STUD SURF SCI CATAL, V84, P1375
[10]  
ICHIKAWA S, 1984, ACS SYM SER, V248, P439