Cryogenic spectroscopy of ultra-low density colloidal lead chalcogenide quantum dots on chip-scale optical cavities towards single quantum dot near-infrared cavity QED

被引：11

作者：

Bose, Ranojoy ^{[1
]}

Gao, Jie ^{[1
]}

McMillan, James F. ^{[1
]}

Williams, Alex D. ^{[1
]}

Wong, Chee Wei ^{[1
]}

机构：

[1] Columbia Univ, Opt Nanostruct Lab, Ctr Integrated Sci & Engn, New York, NY 10027 USA

来源：

OPTICS EXPRESS | 2009年 / 17卷 / 25期

关键词：

PBS NANOCRYSTALS; ENERGY-TRANSFER; PHOTON SOURCE; TEMPERATURE; SYSTEM; MICROCAVITIES; NANOCAVITY; EMISSION; SOLIDS; STATE;

D O I：

10.1364/OE.17.022474

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We present evidence of cavity quantum electrodynamics from a sparse density of strongly quantum-confined Pb-chalcogenide nanocrystals (between 1 and 10) approaching single-dot levels on moderately high-Q mesoscopic silicon optical cavities. Operating at important near-infrared (1500-nm) wavelengths, large enhancements are observed from devices and strong modifications of the QD emission are achieved. Saturation spectroscopy of coupled QDs is observed at 77K, highlighting the modified nanocrystal dynamics for quantum information processing. (C) 2009 Optical Society of America

引用

页码：22474 / 22483

页数：10

共 56 条

[1]

AKIMOV AI, 1985, SOLID STATE COMMUN, V56, P921

[2] Confinement effects in PbSe quantum wells and nanocrystals [J].

Allan, G ;

Delerue, C .

PHYSICAL REVIEW B, 2004, 70 (24) :1-9

[3] The excitonic exchange splitting and radiative lifetime in PbSe quantum dots [J].

An, J. M. ;

Franceschetti, A. ;

Zunger, A. .

NANO LETTERS, 2007, 7 (07) :2129-2135

[4] Pure emitter dephasing: A resource for advanced solid-state single-photon sources [J].

Auffeves, Alexia ;

Gerard, Jean-Michel ;

Poizat, Jean-Philippe .

PHYSICAL REVIEW A, 2009, 79 (05)

[5] Deterministic coupling of single quantum dots to single nanocavity modes [J].

Badolato, A ;

Hennessy, K ;

Atatüre, M ;

Dreiser, J ;

Hu, E ;

Petroff, PM ;

Imamoglu, A .

SCIENCE, 2005, 308 (5725) :1158-1161

[6]

BOSE R, 2005, P SOC PHOTO-OPT INS

[7] Temperature-tuning of near-infrared monodisperse quantum dot solids at 1.5 μm for controllable Forster energy transfer [J].

Bose, Ranojoy ;

McMillan, James F. ;

Gao, Jie ;

Rickey, Kelly M. ;

Chen, Chariton J. ;

Talapin, Dmitri V. ;

Murray, Christopher B. ;

Wong, Chee Wei .

NANO LETTERS, 2008, 8 (07) :2006-2011

[8] Weak coupling interactions of colloidal lead sulphide nanocrystals with silicon photonic crystal nanocavities near 1.55 μm at room temperature [J].

Bose, Ranojoy ;

Yang, Xiaodong ;

Chatterjee, Rohit ;

Gao, Jie ;

Wong, Chee Wei .

APPLIED PHYSICS LETTERS, 2007, 90 (11)

[9] Colloidal CdSe/ZnS quantum dots as single-photon sources [J].

Brokmann, X ;

Messin, G ;

Desbiolles, P ;

Giacobino, E ;

Dahan, M ;

Hermier, JP .

NEW JOURNAL OF PHYSICS, 2004, 6 :1-8

[10] ELECTRON ELECTRON AND ELECTRON-HOLE INTERACTIONS IN SMALL SEMICONDUCTOR CRYSTALLITES - THE SIZE DEPENDENCE OF THE LOWEST EXCITED ELECTRONIC STATE [J].

BRUS, LE .

JOURNAL OF CHEMICAL PHYSICS, 1984, 80 (09) :4403-4409

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