Melting of incommensurate-ferroelectric phase with magnetic field in multiferroic TbMnO3

被引:31
作者
Argyriou, D. N.
Aliouane, N.
Strempfer, J.
Zegkinoglou, I.
Bohnenbuck, B.
Habicht, K.
Zimmermann, M. V.
机构
[1] Hahn Meitner Inst Berlin GmbH, D-14109 Berlin, Germany
[2] Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany
[3] DESY, HASYLAB, D-22603 Hamburg, Germany
来源
PHYSICAL REVIEW B | 2007年 / 75卷 / 02期
关键词
D O I
10.1103/PhysRevB.75.020101
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have investigated the reentrant ferroelectric behavior of TbMnO3 under a c-axis-aligned magnetic field (H parallel to c) using neutron and x-ray single-crystal diffraction. We find that below T-N=41 K and at high field the incommensurate ordering of Mn spins melts and coincides with the disappearance of ferroelectricity. The paraelectric phase which emerges is characterized by a simple commensurate antiferomagnetic ordering. We suggest that the reentrance of ferroelectricity at low temperatures and high magnetic field coincides with the development of incommensurate Mn- and Tb-spin ordering.
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页数:4
相关论文
共 13 条
[1]   Field-induced linear magnetoelastic coupling in multiferroic TbMnO3 -: art. no. 020102 [J].
Aliouane, N ;
Argyriou, DN ;
Strempfer, J ;
Zegkinoglou, I ;
Landsgesell, S ;
Zimmermann, MV .
PHYSICAL REVIEW B, 2006, 73 (02)
[2]   THEORY OF THE ROLE OF COVALENCE IN THE PEROVSKITE-TYPE MANGANITES [LA,M(II)]MNO3 [J].
GOODENOUGH, JB .
PHYSICAL REVIEW, 1955, 100 (02) :564-573
[3]   Ferroelectricity and giant magnetocapacitance in perovskite rare-earth manganites [J].
Goto, T ;
Kimura, T ;
Lawes, G ;
Ramirez, AP ;
Tokura, Y .
PHYSICAL REVIEW LETTERS, 2004, 92 (25) :257201-1
[4]  
Hill NA, 2000, J PHYS CHEM B, V104, P6694, DOI [10.1021/jp000114x, 10.1021/jpc00114x]
[5]   Magnetic structure of TbMnO3 by neutron diffraction -: art. no. 012401 [J].
Kajimoto, R ;
Yoshizawa, H ;
Shintani, H ;
Kimura, T ;
Tokura, Y .
PHYSICAL REVIEW B, 2004, 70 (01) :012401-1
[6]  
KATSURA H, IN PRESS PHYS REV LE
[7]   Magnetic inversion symmetry breaking and ferroelectricity in TbMnO3 -: art. no. 087206 [J].
Kenzelmann, M ;
Harris, AB ;
Jonas, S ;
Broholm, C ;
Schefer, J ;
Kim, SB ;
Zhang, CL ;
Cheong, SW ;
Vajk, OP ;
Lynn, JW .
PHYSICAL REVIEW LETTERS, 2005, 95 (08)
[8]   Magnetoelectric phase diagrams of orthorhombic RMnO3 (R=Gd, Tb, and Dy) [J].
Kimura, T ;
Lawes, G ;
Goto, T ;
Tokura, Y ;
Ramirez, AP .
PHYSICAL REVIEW B, 2005, 71 (22)
[9]   Distorted perovskite with eg1 configuration as a frustrated spin system -: art. no. 060403 [J].
Kimura, T ;
Ishihara, S ;
Shintani, H ;
Arima, T ;
Takahashi, KT ;
Ishizaka, K ;
Tokura, Y .
PHYSICAL REVIEW B, 2003, 68 (06)
[10]   Magnetic control of ferroelectric polarization [J].
Kimura, T ;
Goto, T ;
Shintani, H ;
Ishizaka, K ;
Arima, T ;
Tokura, Y .
NATURE, 2003, 426 (6962) :55-58