In-gap spin excitations and finite triplet lifetimes in the dilute singlet ground state system SrCu2-xMgx(BO3)2

被引:22
作者
Haravifard, S. [1 ]
Dunsiger, S. R.
El Shawish, S.
Gaulin, B. D.
Dabkowska, H. A.
Telling, M. T. F.
Perring, T. G.
Bonca, J.
机构
[1] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada
[2] Jozef Stefan Inst, SI-1000 Ljubljana, Slovenia
[3] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada
[4] Rutherford Appleton Lab, ISIS Pulsed Neutron Facil, Didcot OX11 0QX, Oxon, England
[5] Univ Ljubljana, Fac Math & Phys, SI-1000 Ljubljana, Slovenia
关键词
D O I
10.1103/PhysRevLett.97.247206
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
High resolution neutron scattering measurements on a single crystal of SrCu2-xMgx(BO3)(2) with x similar to 0.05 reveal the presence of new spin excitations within the gap of this quasi-two-dimensional, singlet ground state system. The application of a magnetic field induces Zeeman-split states associated with S=1/2 unpaired spins which are antiferromagnetically correlated with the bulk singlet. Substantial broadening of both the one- and two-triplet excitations in the doped single crystal is observed, as compared with pure SrCu2(BO3)(2). Theoretical calculations using a variational algorithm and a single quenched magnetic vacancy on an infinite lattice are shown to qualitatively account for these effects.
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页数:4
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