Femtosecond microscopy of surface plasmon polariton wave packet evolution at the silver/vacuum interface

被引:240
作者
Kubo, Atsushi
Pontius, Niko
Petek, Hrvoje [1 ]
机构
[1] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA
[2] Univ Pittsburgh, Petersen Inst NanoSci & Engn, Pittsburgh, PA 15260 USA
[3] Japan Sci & Technol Agcy, PRESTO, Kawaguchi, Saitama, Japan
关键词
D O I
10.1021/nl0627846
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A movie of the dispersive and dissipative propagation of surface plasmon polariton (SPP) wave packets at a silver/vacuum interface is recorded by the interferometric time-resolved photoemission electron microscopy with 60 nm spatial resolution and 330 as frame interval. The evolution of SPP wave packets is imaged through a two-path interference created by a pair of 10 fs phase correlated pump-probe light pulses at 400 nm. The wave packet evolution is simulated using the complex dielectric function of silver.
引用
收藏
页码:470 / 475
页数:6
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