Expanding applications of SERS through versatile nanomaterials engineering

被引：423

作者：

Cardinal, M. Fernanda ^{[1
]}

Ende, Emma Vander ^{[1
]}

Hackler, Ryan A. ^{[1
]}

McAnally, Michael O. ^{[1
]}

Stair, Peter C. ^{[1
]}

Schatz, George C. ^{[1
]}

Van Duyne, Richard P. ^{[1
]}

机构：

[1] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA

来源：

CHEMICAL SOCIETY REVIEWS | 2017年 / 46卷 / 13期

基金：

美国国家科学基金会;

关键词：

ENHANCED RAMAN-SPECTROSCOPY; POLYCYCLIC AROMATIC-HYDROCARBONS; SELF-ASSEMBLED MONOLAYERS; ATOMIC LAYER DEPOSITION; DISTANCE DEPENDENCE; GOLD NANOPARTICLES; UV-SERS; SMALL MOLECULES; BINDING-SITES; IN-VIVO;

D O I：

10.1039/c7cs00207f

中图分类号：

O6 [化学];

学科分类号：

070301 [无机化学];

摘要：

Surface-enhanced Raman scattering (SERS) spectroscopy has evolved into a cross-disciplinary analytical technique by unveiling relevant chemical, biological, material, and structural information. The focus of this review is on two critical properties for successfully expanding applications of SERS spectroscopy: quality of the plasmonic substrate and molecule localization to the substrate. In this review, we discuss recent work on quantifying SERS distance dependence, key factors for substrate characterization and performance evaluation, expansion of SERS applications through substrate development for UV plasmonics and short-distance capture strategies for optimizing analyte-surface structures. After surveying the recent developments of these seemingly disparate fields, we suggest new research directions that may originate from a synergistic blend of all the herein discussed topics. Finally, we discuss major challenges and open questions related to the application of SERS for understanding of chemical processes at the nanoscale, with special interest on in situ catalysts and biosensing.

引用

页码：3886 / 3903

页数：18

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