New particle formation in Beijing, China:: Statistical analysis of a 1-year data set

被引:254
作者
Wu, Zhijun
Hu, Min [1 ]
Liu, Shang
Wehner, Birgit
Bauer, Stefan
Ssling, Andreas Ma
Wiedensohler, Alfred
Petaejae, Tuukka
Dal Maso, Miikka
Kulmala, Markku
机构
[1] Peking Univ, Coll Environm Sci, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100871, Peoples R China
[2] Leibniz Inst Tropospher Res, D-04318 Leipzig, Germany
[3] Univ Helsinki, Dept Phys Sci, Div Atmospher Sci, FI-00014 Helsinki, Finland
关键词
D O I
10.1029/2006JD007406
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Particle number size distributions between 3 nm and 10 mm were measured in Beijing, China. New particle formation events were observed on around 40% of the measurement days from March 2004 to February 2005 and were generally observed under low relative humidity and sunny conditions. Though occurring during all seasons, new particle formation events had highest frequency in spring and lowest frequency in summer. Events were classified as "clean'' or "polluted'' groups mainly according to the condensational sink and the local wind. The formation rate range was from 3.3 to 81.4 cm(-3) s(-1). The growth rate varied from 0.1 to 11.2 nm h(-1). The seasonal variation of condensable vapor concentration showed the highest values during summer months due to enhanced photochemical and biological activities as well as stagnant air masses preventing exchange with cleaner air.
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页数:10
相关论文
共 33 条
[1]   Observations of new particle formation in urban air [J].
Alam, A ;
Shi, JP ;
Harrison, RM .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D3)
[2]   New particle formation in the continental boundary layer: Meteorological and gas phase parameter influence [J].
Birmili, W ;
Wiedensohler, A .
GEOPHYSICAL RESEARCH LETTERS, 2000, 27 (20) :3325-3328
[3]   The Hohenpeissenberg aerosol formation experiment (HAFEX):: a long-term study including size-resolved aerosol, H2SO4, OH, and monoterpenes measurements [J].
Birmili, W ;
Berresheim, H ;
Plass-Dülmer, C ;
Elste, T ;
Gilge, S ;
Wiedensohler, A ;
Uhrner, U .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2003, 3 :361-376
[4]  
Dal Maso M, 2005, BOREAL ENVIRON RES, V10, P323
[5]   Measurements of Mexico City nanoparticle size distributions:: Observations of new particle formation and growth -: art. no. L10102 [J].
Dunn, MJ ;
Jiménez, JL ;
Baumgardner, D ;
Castro, T ;
McMurry, PH ;
Smith, JN .
GEOPHYSICAL RESEARCH LETTERS, 2004, 31 (10) :L101021-4
[6]   The investigations of aerosol particle formation in urban background area of Helsinki [J].
Hameri, K ;
Kulmala, M ;
Aalto, P ;
Leszczynski, K ;
Visuri, R ;
Hamekoski, K .
ATMOSPHERIC RESEARCH, 1996, 41 (3-4) :281-298
[7]   PROPERTIES OF THE LOG-NORMAL PARTICLE-SIZE DISTRIBUTION [J].
HEINTZENBERG, J .
AEROSOL SCIENCE AND TECHNOLOGY, 1994, 21 (01) :46-48
[8]  
Kerminen VM, 2001, J GEOPHYS RES-ATMOS, V106, P24119, DOI 10.1029/2001JD000322
[9]   Effect of NO2 on particle formation in SO2 /H2O/air mixtures by ion-induced and homogeneous nucleation [J].
Kim, CS ;
Adachi, M ;
Okuyama, K ;
Seinfeld, JH .
AEROSOL SCIENCE AND TECHNOLOGY, 2002, 36 (09) :941-952
[10]   Ternary nucleation of H2SO4, NH3, and H2O in the atmosphere [J].
Korhonen, P ;
Kulmala, M ;
Laaksonen, A ;
Viisanen, Y ;
McGraw, R ;
Seinfeld, JH .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D21) :26349-26353