On the significance of regional trace gas distributions as derived from aircraft campaigns in PEM-West A and B

被引:9
作者
Ehhalt, DH
Rohrer, F
Kraus, AB
Prather, MJ
Blake, DR
Rowland, FS
机构
[1] Forschungszentrum Julich, Inst Atmosphar Chem, D-52425 Julich, Germany
[2] Univ Calif Irvine, Dept Chem, Irvine, CA 92717 USA
[3] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92717 USA
关键词
D O I
10.1029/97JD01498
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
With the help of a chemical transport model we calculate the global distributions of three synthetic tracers with uniform emission rates over the continents, zero emissions over the ocean, and constant lifetimes of 5, 20, and 100 days. These distributions serve as a first approximation to those of the lower alkanes and are analyzed in detail for the region between 115 degrees E and 155 degrees E longitude, 0 degrees N and 56 degrees N latitude, within which the Pacific Exploratory Mission-West (PEM-West) A and B campaigns took place. We show that the longitudinally averaged latitude by altitude distributions of the tracers over that domain obtained from sampling the model data along the flight tracks closely represent those obtained from complete averages over the full data sets for the months March and September when the campaigns took place. We further show that for each campaign the modeled distributions closely resemble those measured for ethane and propane, although these distributions change significantly between the two seasons. Taken together, this demonstrates that the average distributions of ethane and propane measured during PEM-West A and B describe reasonably well the true pattern of these gases between 0 degrees N and 50 degrees N latitude and 115 degrees E and 155 degrees E longitude in both seasons, despite incomplete and irregular sampling of that domain. In turn, the measured distributions can be used to test the model, mainly for correct parameterization of transport.
引用
收藏
页码:28333 / 28351
页数:19
相关论文
共 11 条
  • [1] PEM-West A: Meteorological overview
    Bachmeier, AS
    Newell, RE
    Zhu, Y
    Blake, DR
    Browell, EV
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D1) : 1655 - 1677
  • [2] Three-dimensional distribution of nonmenthane hydrocarbons and halocarbons over the northwestern Pacific during the 1991 Pacific Exploratory Mission (PEM-West A)
    Blake, DR
    Chen, TY
    Smith, TY
    Wang, CJL
    Wingenter, OW
    Blake, NJ
    Rowland, FS
    Mayer, EW
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D1) : 1763 - 1778
  • [3] GREGORY GL, 1995, TM110193 NASA LANGL
  • [4] HANSEN J, 1983, MON WEATHER REV, V111, P609, DOI 10.1175/1520-0493(1983)111<0609:ETDGMF>2.0.CO
  • [5] 2
  • [6] Hydrocarbon ratios during PEM-WEST A: A model perspective
    McKeen, SA
    Liu, SC
    Hsie, EY
    Lin, X
    Bradshaw, JD
    Smyth, S
    Gregory, GL
    Blake, DR
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D1) : 2087 - 2109
  • [7] CHEMISTRY OF THE GLOBAL TROPOSPHERE - FLUOROCARBONS AS TRACERS OF AIR MOTION
    PRATHER, M
    MCELROY, M
    WOFSY, S
    RUSSELL, G
    RIND, D
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1987, 92 (D6) : 6579 - 6613
  • [8] NUMERICAL ADVECTION BY CONSERVATION OF 2ND-ORDER MOMENTS
    PRATHER, MJ
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1986, 91 (D6) : 6671 - 6681
  • [9] ATMOSPHERIC TRENDS AND LIFETIME OF CH3CCL3 AND GLOBAL OH CONCENTRATIONS
    PRINN, RG
    WEISS, RF
    MILLER, BR
    HUANG, J
    ALYEA, FN
    CUNNOLD, DM
    FRASER, PJ
    HARTLEY, DE
    SIMMONDS, PG
    [J]. SCIENCE, 1995, 269 (5221) : 187 - 192
  • [10] THE TROPOSPHERIC DISTRIBUTION AND BUDGET OF ETHANE
    RUDOLPH, J
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1995, 100 (D6) : 11369 - 11381