Time-dependent density functional theory beyond the adiabatic local density approximation

被引:216
作者
Vignale, G [1 ]
Ullrich, CA [1 ]
Conti, S [1 ]
机构
[1] SCUOLA NORMALE SUPER PISA,I-56126 PISA,ITALY
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.79.4878
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
In the current density functional theory of linear and nonlinear time-dependent phenomena, the treatment of exchange and correlation beyond the level of the adiabatic local density approximation is shown to lead to the appearance of viscoelastic stresses in the electron fluid. Complex and frequency-dependent viscosity/elasticity coefficients are microscopically derived and expressed in terms of properties of the homogeneous electron gas, As a first consequence of this formalism, we provide an explicit formula for the linewidths of collective excitations in electronic systems.
引用
收藏
页码:4878 / 4881
页数:4
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