Simultaneous removal of NOx and SO2 from coal boiler flue gases by DC corona discharge ammonia radical shower systems:: pilot plant tests

被引:69
作者
Chang, JS
Urashima, K
Tong, YX
Liu, WP
Wei, HY
Yang, FM
Liu, XJ
机构
[1] McMaster Univ, Dept Engn Phys, Hamilton, ON L8S 4M1, Canada
[2] State Environm Protect Gen Agcy, Safety & Environm Protect Res Inst, Wuhan, Peoples R China
基金
加拿大自然科学与工程研究理事会;
关键词
non-thermal plasma; flow stabilized corona discharge; radical injection; coal boiler flue gases; NOx and SO2; ammonia radical; flue gas;
D O I
10.1016/S0304-3886(02)00168-7
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Pilot scale tests were conducted for simultaneous removal of NOx and SO2 from coal boiler flue gases by corona discharge induced ammonia radical injection techniques, i.e. the corona radical shower system. Tests were conducted for the flue gas rate from 1000 to 1500 Nm(3)/h, the gas temperature from 62degreesC to 80degreesC, the ammonia-to-total acid gas molecule ratio from 0.88 to 1.3, applied voltage from 0 to 25 kV and NO initial concentration from 53 to 93 ppm. for a fixed SO2 of 800 ppm. The results show that SO2 removal increases with increasing ammonia radical injection rate and non-monotonically depends on in-put electrical power. The NOx removal increases with increasing in-put electrical power and ammonia radical injection rate. Approximately 9 kg Of SO2 were removed by 1 kWh of energy input with 99% Of SO2 removal, while approximately 125 g of NOx was removed by 1 kWh of energy input with 75% of removal efficiency. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:313 / 323
页数:11
相关论文
共 20 条
[1]  
Chang J. S., 1988, Conference Record of the 1988 Industry Applications Society Annual Meeting (IEEE Cat. No.88CH2565-0), P1628, DOI 10.1109/IAS.1988.25276
[2]   Growth and survival of Escherichia coli O157:H7 during the fermentation and storage of diluted cultured milk drink [J].
Chang, JH ;
Chou, CC ;
Li, CF .
FOOD MICROBIOLOGY, 2000, 17 (06) :579-587
[3]   CORONA DISCHARGE PROCESSES [J].
CHANG, JS ;
LAWLESS, PA ;
YAMAMOTO, T .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 1991, 19 (06) :1152-1166
[4]   Live E. coli cells to treat uremia [J].
T.M.S. Chang .
Nature Medicine, 1997, 3 (1) :3-4
[5]   COMBINED REMOVAL OF SO2, NOX, AND FLY-ASH FROM SIMULATED FLUE-GAS USING PULSED STREAMER CORONA [J].
CLEMENTS, JS ;
MIZUNO, A ;
FINNEY, WC ;
DAVIS, RH .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 1989, 25 (01) :62-69
[6]   INDUSTRIAL EXPERIMENTS ON PULSE CORONA SIMULTANEOUS REMOVAL OF NOX AND SO2 FROM FLUE-GAS [J].
DINELLI, G ;
CIVITANO, L ;
REA, M .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 1990, 26 (03) :535-541
[7]   Energy policy and politics in China [J].
Hood, M ;
Sweet, W .
IEEE SPECTRUM, 1999, 36 (11) :34-38
[8]   Semipilot plant pulse energized cold-precharger electrostatic precipitator tests for collection of moderately high resistivity flyash particles [J].
Jayaram, S ;
Castle, GSP ;
Chang, JS ;
Berezin, AA ;
Looy, PC ;
Mangal, R ;
Mozes, MS .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 1996, 32 (04) :851-857
[9]   Reduction of NOx from flue gas by corona discharge activated ammonia radical showers [J].
Kanazawa, S ;
Chang, JS ;
Round, GF ;
Sheng, G ;
Ohkubo, T ;
Nomoto, Y ;
Adachi, T .
COMBUSTION SCIENCE AND TECHNOLOGY, 1998, 133 (1-3) :93-105
[10]   PILOT-PLANT EXPERIMENT ON THE TREATMENT OF EXHAUST-GAS FROM A SINTERING MACHINE BY ELECTRON-BEAM IRRADIATION [J].
KAWAMURA, K ;
AOKI, S ;
KIMURA, H ;
ADACHI, K ;
KAWAMURA, K ;
KATAYAMA, T ;
KENGAKU, K ;
SAWADA, Y .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1980, 14 (03) :288-293