New inter-Rydberg transitions of NO revealed by the laser induced amplified spontaneous emission

被引：15

作者：

Ogi, Y

Sugita, A

Suzuki, H

Tanaka, Y

Tsukiyama, K ^{[1
]}

机构：

[1] Sci Univ Tokyo, Fac Sci, Dept Chem, Shinjuku Ku, Tokyo 162, Japan

[2] Harima Res Estab, RIKEN, Sayo, Hyogo, Japan

来源：

JOURNAL OF CHEMICAL PHYSICS | 1998年 / 108卷 / 03期

关键词：

D O I：

10.1063/1.475453

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Amplified spontaneous emission (ASE) from single rotational levels of Rydberg states, 4p sigma M (2) Sigma(+), 4p pi K (2) Pi, 5s sigma S (2) Sigma(+), 4d sigma O (2) Sigma(+), 4d pi O' (2) Pi, 5p sigma R (2) Sigma(+), and 5p pi Q (2) Pi of NO molecules has been investigated through optical-optical double resonance excitation via the A (2) Sigma(+) state. Several new inter-Rydberg transitions were identified in the midinfrared region. The rotational structure in dispersed ASE spectra was resolved completely, which provided detailed information on cascading radiative relaxation processes among Rydberg states. (C) 1998 American Institute of Physics. [S0021-9606(98)02603-8].

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页码：900 / 906

页数：7

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