Absolute measurement of the optical polarizability of C60

被引:78
作者
Ballard, A [1 ]
Bonin, K [1 ]
Louderback, J [1 ]
机构
[1] Wake Forest Univ, Dept Phys, Winston Salem, NC 27109 USA
关键词
D O I
10.1063/1.1290472
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We report on a new optical technique that uses light forces and a time-of-flight spectrometer to make absolute measurements of cluster polarizabilities. This is also the first accurate report of an ac polarizability measurement of a condensable cluster in the gas phase. We have determined the optical polarizability of C-60 at the fundamental wavelength of a Nd:YAG laser (1.064 mu m) to be alpha=79 +/- 4 Angstrom(3). (C) 2000 American Institute of Physics. [S0021- 9606(00)01038-2].
引用
收藏
页码:5732 / 5735
页数:4
相关论文
共 17 条
[1]   Static dipole polarizability of small mixed sodium-lithium clusters [J].
Antoine, R ;
Rayane, D ;
Allouche, AR ;
Frécon, MA ;
Benichou, E ;
Dalby, FW ;
Dugourd, P ;
Broyer, M ;
Guet, C .
JOURNAL OF CHEMICAL PHYSICS, 1999, 110 (12) :5568-5577
[2]   Direct measurement of the electric polarizability of isolated C60 molecules [J].
Antoine, R ;
Dugourd, P ;
Rayane, D ;
Benichou, E ;
Broyer, M ;
Chandezon, F ;
Guet, C .
JOURNAL OF CHEMICAL PHYSICS, 1999, 110 (19) :9771-9772
[3]   Measurement of static electric dipole polarizabilities of lithium clusters: Consistency with measured dynamic polarizabilities [J].
Benichou, E ;
Antoine, R ;
Rayane, D ;
Vezin, B ;
Dalby, FW ;
Dugourd, P ;
Broyer, M ;
Ristori, C ;
Chandezon, F ;
Huber, BA ;
Rocco, JC ;
Blundell, SA ;
Guet, C .
PHYSICAL REVIEW A, 1999, 59 (01) :R1-R4
[4]  
Bonin K. D., 1997, ELECT DIPOLE POLARIZ
[5]   THEORY OF THE LIGHT-FORCE TECHNIQUE FOR MEASURING POLARIZABILITIES [J].
BONIN, KD ;
KADARKALLEN, MA .
PHYSICAL REVIEW A, 1993, 47 (02) :944-960
[6]   LARGE ION VOLUME TIME-OF-FLIGHT MASS-SPECTROMETER WITH POSITION-SENSITIVE AND VELOCITY-SENSITIVE DETECTION CAPABILITIES FOR CLUSTER BEAMS [J].
DEHEER, WA ;
MILANI, P .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1991, 62 (03) :670-677
[7]   NONJELLIUM-TO-JELLIUM TRANSITION IN ALUMINUM CLUSTER POLARIZABILITIES [J].
DEHEER, WA ;
MILANI, P ;
CHATELAIN, A .
PHYSICAL REVIEW LETTERS, 1989, 63 (26) :2834-2836
[8]   THE PHYSICS OF SIMPLE METAL-CLUSTERS - EXPERIMENTAL ASPECTS AND SIMPLE-MODELS [J].
DEHEER, WA .
REVIEWS OF MODERN PHYSICS, 1993, 65 (03) :611-676
[9]   OPTICAL-PROPERTIES OF C-60-BASED AND C-70-BASED SOLID FILMS [J].
EKLUND, PC ;
RAO, AM ;
WANG, Y ;
ZHOU, P ;
WANG, KA ;
HOLDEN, JM ;
DRESSELHAUS, MS ;
DRESSELHAUS, G .
THIN SOLID FILMS, 1995, 257 (02) :211-232
[10]   FULLERENE TRIPLET-STATE PRODUCTION AND DECAY - R2PI PROBES OF C60 AND C70 IN A SUPERSONIC BEAM [J].
HAUFLER, RE ;
WANG, LS ;
CHIBANTE, LPF ;
JIN, CM ;
CONCEICAO, J ;
CHAI, Y ;
SMALLEY, RE .
CHEMICAL PHYSICS LETTERS, 1991, 179 (5-6) :449-454